Reactive high-spin iron(IV)-oxo sites through dioxygen activation in a metal–organic framework

已完结 10 由 x123 发布于 2025/4/19 21:10:35

DOI:10.1126/science.add7417
作者：Kaipeng Hou,?Jonas B?rgel,?Henry Z. H. Jiang,?Daniel J. SantaLucia,?Hyunchul Kwon,?Hao Zhuang,?Khetpakorn Chakarawet,?Rachel C. Rohde,?Jordan W. Taylor,?Chaochao Dun,?Maria V. Paley,?Ari B. Turkiewicz
文献类型：期刊论文
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American Association for the Advancement of Science (AAAS)

Abstract：In nature, nonheme iron enzymes use dioxygen to generate high-spin iron(IV)=O species for a variety of oxygenation reactions. Although synthetic chemists have long sought to mimic this react

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