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Quenching high-temperature phase in Cu–Sn alloy system by femtosecond and picosecond laser irradiation 用飞秒和皮秒激光辐照淬灭铜锡合金体系中的高温相
IF 2.5 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-22 DOI: 10.1007/s00339-024-07997-4
Taketo Furuichi, Hiroto Seki, Taiyoh Kawano, Keisuke Takabayashi, Tsubasa Endo, Eibon Tsuchiya, Makoto Yamaguchi, Yohei Kobayashi, Tatsuya Okada, Takuro Tomita

This study investigated the dependence of irradiation fluence and pulse duration on the non–thermal alloying of Cu and Sn through laser irradiation. Femtosecond and picosecond laser irradiation were applied to the GaN part of a bilayer of Cu and Sn deposited on GaN. The laser beam operated at a wavelength and repetition rate of 1030 nm and 1 MHz, respectively, with pulse durations of 0.65 and 38 ps. Subsequently, the irradiated samples were thinned using a focused ion beam, and the cross-sections were examined with transmission electron microscopy. The lattice constants of the resultant phases were identified from selected area diffraction patterns. In data analysis, we identified the phases as β-Sn and ε-phases first, if discernible within a 5% error margin, employing high-temperature phases when identification was not possible. In the irradiated area, only Cu and Sn were detected under a lower fluence and shorter pulse duration. However, δ-phases, which are alloys of Cu and Sn, formed at relatively higher fluences and longer pulse durations. This high-temperature phase, unique to picosecond laser irradiation, cannot be obtained through conventional thermodynamic processes, highlighting the unique capabilities of laser-induced processing in creating novel alloy phases. These findings advance our understanding of laser-material interactions and provides a foundation for developing advanced materials with tailored properties for various applications.

本研究探讨了辐照通量和脉冲持续时间对通过激光辐照实现铜和锡非热合金化的影响。对沉积在氮化镓上的铜和锡双层层的氮化镓部分进行了飞秒和皮秒激光辐照。激光束的波长和重复频率分别为 1030 nm 和 1 MHz,脉冲持续时间分别为 0.65 和 38 ps。随后,使用聚焦离子束对辐照样品进行减薄,并使用透射电子显微镜对横截面进行检测。从选定的区域衍射图样中确定了所产生相的晶格常数。在数据分析中,如果能在 5%误差范围内辨别出相,我们首先将其识别为 β-Sn 相和ε相,如果无法识别,则采用高温相。在辐照区域,在较低的通量和较短的脉冲持续时间下,只能检测到铜和锡。然而,在相对较高的通量和较长的脉冲持续时间下,形成了铜、锡合金的δ相。这种高温相是皮秒激光辐照所特有的,无法通过传统的热力学过程获得,凸显了激光诱导加工在创造新型合金相方面的独特能力。这些发现加深了我们对激光与材料相互作用的理解,为开发具有定制特性的先进材料以用于各种应用奠定了基础。
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引用次数: 0
Effect of thiourea concentration on the structural, optical and photoelectric properties of ZnO/ZnS/PVC composite films used as flexible UV photodetectors 硫脲浓度对用作柔性紫外线光电探测器的 ZnO/ZnS/PVC 复合薄膜的结构、光学和光电特性的影响
IF 2.5 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-22 DOI: 10.1007/s00339-024-07965-y
Hanane Houadsi, Sara Benzitouni, Mourad Zaabat, Louardi Remache, Abdelhakim Mahdjoub

In this work, a new design of flexible photodetectors based on ZnO/ZnS/PVC composite films was realized using polyvinyl chloride as the polymer substrate. ZnO/ZnS composites were successfully synthesized by a hydrothermal method using a mixture of zinc acetate and thiourea, resulting in the formation of microspheres with a core- shell structure. The effect of thiourea concentration as sulfur source (0.2, 0.4, and 0.6 M) on the physical properties of ZnO/ZnS composites was investigated. XRD patterns and FTIR spectra demonstrated a successful fabrication of ZnO and ZnS composites. In addition, the particle size, morphology, elemental composition and the bandgap energy of ZnO/ZnS were studied through the utilization of SEM, EDS and UV-visible spectrophotometer. Finally, the effect of thiourea on the performance of UV photodetectors based on ZnO/ZnS/PVC composite films was investigated using I–V characteristics under dark and UV light conditions. The results showed that the photodetection of the samples improved with increasing thiourea concentration. In particular, the UV photodetector based on PVC-ZSO-3 exhibits a higher photocurrent (2.55 nA), responsivity (0.187 µA/W) and detectivity (5.18 × 106 Jones) than other samples. This gives the impression that the polymer as an insulating material has a promising future as a flexible photodetector worth exploiting.

本研究以聚氯乙烯为聚合物基底,实现了基于 ZnO/ZnS/PVC 复合薄膜的柔性光电探测器的新设计。利用醋酸锌和硫脲的混合物,通过水热法成功合成了 ZnO/ZnS 复合材料,形成了具有核壳结构的微球。研究了硫脲浓度作为硫源(0.2、0.4 和 0.6 M)对 ZnO/ZnS 复合材料物理性质的影响。XRD 图谱和傅立叶变换红外光谱表明,ZnO 和 ZnS 复合材料的制备是成功的。此外,还利用 SEM、EDS 和紫外可见分光光度计研究了 ZnO/ZnS 的粒度、形貌、元素组成和带隙能。最后,利用暗光和紫外光条件下的 I-V 特性研究了硫脲对基于 ZnO/ZnS/PVC 复合薄膜的紫外光探测器性能的影响。结果表明,样品的光电探测性能随着硫脲浓度的增加而提高。特别是基于 PVC-ZSO-3 的紫外光检测器比其他样品表现出更高的光电流(2.55 nA)、响应度(0.187 µA/W)和检测度(5.18 × 106 Jones)。这给人的印象是,聚合物作为一种绝缘材料,作为一种灵活的光电探测器,前景广阔,值得开发。
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引用次数: 0
Mode-hop-free synchronous tuning range extension of an uncoated external cavity diode laser based on PZT hysteresis characteristic compensation 基于 PZT 滞后特性补偿的非涂层外腔二极管激光器的无模式跳频同步调谐范围扩展
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-10-22 DOI: 10.1007/s00340-024-08342-6
Yu Zhu, Binbin Qiu, Weidong Li, Zhigang Liu

External cavity diode laser (ECDL) can continuously alter its output optical frequency by tuning the external cavity. Wide mode-hop-free (MHF) range and linear optical frequency tuning are two critical characteristics of the ECDL. However, using an uncoated laser diode (LD) limits the MHF range due to the influence of internal cavity formed by the LD. To obtain linear optical frequency, a triangular wave voltage is generally used to scan the external cavity. Nevertheless, the inherent hysteresis characteristic of piezoelectric transducer (PZT) in the external cavity introduces nonlinearity in the optical frequency. The limited MHF range and nonlinear optical frequency can greatly affect the performance and accuracy of applications with uncoated ECDL as the light source. Therefore, it is crucial to address these two issues of uncoated ECDL. This study introduces a hybrid method incorporating synchronous tuning with proportional-integral-derivative (PID) feedback control. Synchronous tuning facilitates simultaneous changes in both the internal and external cavities output modes, thereby extending the MHF range. PID feedback control utilizes the displacement signal of prism in the external cavity to establish a closed-loop control system, compensating for the PZT’s hysteresis. Through PID feedback control, the uncoated ECDL’s optical frequency tuning nonlinearity is effectively suppressed while its MHF range is extended. Experimental results validate the efficacy of this hybrid method within the triangular wave scanning frequency of 50 Hz.

外腔二极管激光器(ECDL)可通过调谐外腔连续改变其输出光频。宽无跳模(MHF)范围和线性光频率调谐是 ECDL 的两个关键特性。然而,使用未涂层激光二极管(LD)会受 LD 形成的内腔影响,从而限制 MHF 范围。为了获得线性光频,通常使用三角波电压来扫描外部空腔。然而,外腔中压电传感器(PZT)固有的滞后特性会给光频带来非线性。有限的 MHF 范围和非线性光频会极大地影响使用未涂层 ECDL 作为光源的应用的性能和精度。因此,解决无涂层 ECDL 的这两个问题至关重要。本研究引入了一种混合方法,将同步调节与比例-积分-派生(PID)反馈控制相结合。同步调谐有助于同时改变内腔和外腔的输出模式,从而扩大 MHF 范围。PID 反馈控制利用外腔棱镜的位移信号建立闭环控制系统,对 PZT 的滞后进行补偿。通过 PID 反馈控制,未涂层 ECDL 的光学频率调谐非线性得到了有效抑制,同时其 MHF 范围也得到了扩展。实验结果验证了这种混合方法在 50 Hz 三角波扫描频率范围内的有效性。
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引用次数: 0
A polar diatomic molecule under a high-frequency laser field: classical analytical solution 高频激光场下的极性二原子分子:经典解析解
IF 2.8 3区 物理与天体物理 Q2 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-10-22 DOI: 10.1140/epjp/s13360-024-05727-6
N. Kryukov, E. Oks

Dynamics of a polar diatomic molecule (represented as the oscillating rotator model) under external fields is the most fundamental problem and the testbed in molecular physics—analogously to the dynamics of hydrogenic atom (represented as the model of an electron in the Coulomb field) under external fields being the most fundamental problem and the testbed in atomic physics. We present the classical analytical study of the dynamical Stark effect in the oscillating rotator under a high-frequency laser field. We obtain the analytical results by using the method of effective potentials. We demonstrate that under the laser field, the rotation frequency increases, while the oscillation frequency decreases, and the amplitude of the oscillations increases. More significantly, the laser field causes the generation of the second harmonic in the oscillations of this system. This is an important, counterintuitive result in studying this fundamental physical system. We also drew attention to some flaws in the literature on this subject.

极性二原子分子(以振荡转子模型为代表)在外力场作用下的动力学是分子物理学中最基本的问题和试验平台--类似于氢原子(以库仑场中的电子模型为代表)在外力场作用下的动力学是原子物理学中最基本的问题和试验平台。我们介绍了高频激光场下振荡转子中动态斯塔克效应的经典分析研究。我们利用有效势的方法得到了分析结果。结果表明,在激光场作用下,旋转频率增加,振荡频率降低,振荡幅度增大。更重要的是,激光场导致了该系统振荡中二次谐波的产生。这是研究这一基本物理系统的一个重要的反直觉结果。我们还提请大家注意有关这一主题的文献中存在的一些缺陷。
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引用次数: 0
Low-temperature fabrication of high-performance AZO/Ag/WO3 multilayer films for flexible heaters 低温制备用于柔性加热器的高性能 AZO/Ag/WO3 多层薄膜
IF 2.5 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-22 DOI: 10.1007/s00339-024-07993-8
Ke Zhu, Kaiwei Yang

In this study, Al-doped ZnO/Ag/WO3 (AZO/Ag/WO3)multilayer films were fabricated on polyethylene terephthalate (PET) substrates using the magnetron sputtering technique. A two-step magnetron sputtering process was employed to deposit WO3, effectively preventing insulation in the AZO/Ag/WO3 multilayer film caused by silver oxidation. The optical properties of the AZO/Ag/WO3 multilayer films can be adjusted by varying the thickness of AZO and WO3 layers. The optimal AZO/Ag/WO3 multilayer film demonstrates a maximum figure-of-merit of 1.74 × 10− 2 Ω−1, with an average visible light transmittance of 81.1% and a sheet resistance of 7.04 Ω sq− 1. When applied in transparent flexible heaters, the AZO/Ag/WO3 multilayer films exhibit rapid thermal response, stable and controllable heating performance at low operating voltage, indicating exceptional thermal properties and high conductivity. The two-step magnetron sputtering deposition of external oxide layers to prevent the oxidation of silver is cost-effective and can be utilized to create high-performance oxide/metal/oxide transparent electrodes.

本研究利用磁控溅射技术在聚对苯二甲酸乙二醇酯(PET)基底上制造了铝掺杂 ZnO/Ag/WO3(AZO/Ag/WO3)多层膜。采用两步磁控溅射工艺沉积 WO3,有效地防止了银氧化导致的 AZO/Ag/WO3 多层膜绝缘。AZO/Ag/WO3 多层薄膜的光学特性可通过改变 AZO 层和 WO3 层的厚度来调节。最佳的 AZO/Ag/WO3 多层薄膜的最大功率为 1.74 × 10- 2 Ω-1,平均可见光透射率为 81.1%,薄片电阻为 7.04 Ω sq-1。当应用于透明柔性加热器时,AZO/Ag/WO3 多层薄膜表现出快速的热响应,在低工作电压下具有稳定、可控的加热性能,显示出卓越的热性能和高导电性。通过两步磁控溅射沉积外部氧化层以防止银氧化的方法具有成本效益,可用于制造高性能的氧化物/金属/氧化物透明电极。
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引用次数: 0
Study of lepton flavor universality and angular distributions in (Drightarrow K^*_{J} (rightarrow Kpi )ell nu _{ell }) Drightarrow K^*_{J} (rightarrow Kpi )ell nu _{ell }) 中轻子味道普遍性和角分布的研究
IF 4.2 2区 物理与天体物理 Q2 PHYSICS, PARTICLES & FIELDS Pub Date : 2024-10-22 DOI: 10.1140/epjc/s10052-024-13456-4
Fei Huang, Ji Xu

The decay of the D meson into multibody final states is a complex process that provides valuable insights into the fundamental interactions within the Standard Model of particle physics. This study focuses on the decay cascade (D^{+}rightarrow K^{*}_{J} ell ^{+}nu rightarrow K^{pm }pi ^{mp } ell ^{+}nu ) where the (K^*_J) resonance encompasses the (K^*(892),K^{*}(1410),K^{*}_0(1430)) states. We employ the helicity amplitude technique to derive the angular distributions for the decay chain, enabling the extraction of one-dimensional and two-dimensional distributions. Utilizing form factors for the (Drightarrow K^*) transition derived from the quark model, we calculate the differential and integrated partial decay widths, explicitly considering the electron and muon masses. Decay branching fractions are calculated, the ratios of the branching fractions are found to be (frac{mathcal {B}r(D^{+}rightarrow K^{*}(892)(rightarrow K ^{-}pi ^{+}) , mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}(892)(rightarrow K ^{-}pi ^{+}) , e^{+}nu _{e})} = 0.975), (frac{mathcal {B}r(D^{+}rightarrow K^{*}(1410)(rightarrow K ^{-}pi ^{+}) , mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}(1410)(rightarrow K ^{-}pi ^{+}) , e^{+}nu _{e})} = 0.714) and (frac{mathcal {B}r(D^{+}rightarrow K^{*}_{0}(1430)(rightarrow K ^{+}pi ^{-}) , mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}_{0}(1430)(rightarrow K ^{+}pi ^{-}) , e^{+}nu _{e})} = 0.774). Results in this work will serve a calibration for the study of (c rightarrow s ) in D meson decays in future and provide useful information towards the understanding of the properties of the (K^{*}) meson, as well as (K pi ) system.

D 介子衰变为多体终态是一个复杂的过程,它为我们了解粒子物理标准模型中的基本相互作用提供了宝贵的视角。这项研究的重点是衰变级联(D^{+}rightarrow K^{*}_{J}ell ^{+}nu rightarrow K^{pm }pi ^{mp }其中共振(K^*_J)包含了(K^*(892),K^{*}(1410),K^{*}_0(1430))态。我们采用螺旋振幅技术来推导衰变链的角度分布,从而能够提取一维和二维分布。利用从夸克模型导出的 (Drightarrow K^*) 转变的形式因子,我们计算了微分和综合部分衰变宽度,明确地考虑了电子和μ介子的质量。我们计算了衰变分支分数,发现分支分数的比值为(frac{mathcal {B}r(D^{+}rightarrow K^{*}(892)(rightarrow K ^{-}pi ^{+}) 、mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}(892)(rightarrow K ^{-}pi ^{+}), e^{+}nu _{e})} = 0.975),(fracmathcal {B}r(D^{+}rightarrow K^{*}(1410)(rightarrow K ^{-}pi ^{+})、mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}(1410)(rightarrow K ^{-}pi ^{+}), e^{+}nu _{e})} = 0.714) and(frac{mathcal {B}r(D^{+}rightarrow K^{*}_{0}(1430)(rightarrow K ^{+}pi ^{-}) 、mu ^{+}nu _{mu })}{mathcal {B}r(D^{+}rightarrow K^{*}_{0}(1430)(rightarrow K ^{+}pi ^{-}) , e^{+}nu _{e})} = 0.774).这项工作的结果将为今后研究D介子衰变中的(c rightarrow s )提供校准,并为理解(K^{*})介子以及(K pi )系统的性质提供有用的信息。
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引用次数: 0
Two pseudo-Goldstone bosons in the Gildener–Weinberg model 吉尔德纳-温伯格模型中的两个伪金石玻色子
IF 4.2 2区 物理与天体物理 Q2 PHYSICS, PARTICLES & FIELDS Pub Date : 2024-10-22 DOI: 10.1140/epjc/s10052-024-13360-x
Parsa Ghorbani

In a dimensionless multi-scalar extension of the Standard Model, Gildener and Weinberg assumed that along a flat direction, there is only one classically massless scalar, known as the scalon, which acquires mass through radiative corrections à la Coleman–Weinberg, while all other scalars remain heavy. In this paper, by introducing a toy model with four scalar degrees of freedom we demonstrate the existence of two scalons along a specific flat direction that we construct. We present the effective potential for the model and provide the masses of the heavy scalars and two radiatively light pseudo-Goldstone bosons.

在标准模型的无量纲多标量扩展中,吉尔德纳和温伯格假定沿平坦方向只有一个经典的无质量标量,即标量子,它通过类似科尔曼-温伯格的辐射修正获得质量,而所有其他标量仍然很重。在本文中,通过引入一个具有四个标量自由度的玩具模型,我们证明了沿着我们构建的特定平面方向存在两个标量子。我们提出了模型的有效势,并提供了重标量和两个辐射轻伪金石玻色子的质量。
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引用次数: 0
Theoretical insights and implications of bouncing cosmology in (f(mathcal {R},textrm{T}^2)) theory f(mathcal{R},textrm{T}^2))理论中反弹宇宙学的理论见解和影响
IF 4.2 2区 物理与天体物理 Q2 PHYSICS, PARTICLES & FIELDS Pub Date : 2024-10-22 DOI: 10.1140/epjc/s10052-024-13473-3
M. Sharif, M. Zeeshan Gul, I. Hashim

In this paper, we explore cosmological bouncing solutions to investigate the cosmic evolution in the framework of energy-momentum squared gravity. We consider flat Friedmann–Robertson–Walker spacetime with a perfect matter distribution. We assume two different functional forms of (f(mathcal {R},T^2)) gravity model to examine the impact of this modified framework in the evolution of the universe. Furthermore, we consider a specific scale factor to investigate different cosmological parameters, analyzing the evolutionary behavior of the universe in this gravity. We also perform stability analysis using the perturbation technique. Our findings indicate that the null energy condition violates at the bounce point and equation of state parameter exhibits characteristics of a quintessence era or phantom regimes. These aspects highlight the complex interplay between energy conditions and stability in bouncing cosmological model. We conclude that the (f(mathcal {R},T^2)) theory successfully provides viable alternatives to the standard cosmological scenarios, offering insights into the early universe and the nature of gravity.

本文探讨了宇宙学弹跳解,以研究能量-动量平方引力框架下的宇宙演化。我们考虑了具有完美物质分布的平坦弗里德曼-罗伯逊-沃克时空。我们假设了两种不同函数形式的(f(mathcal {R},T^2))引力模型,以考察这种修正框架在宇宙演化中的影响。此外,我们还考虑了一个特定的尺度因子来研究不同的宇宙学参数,分析宇宙在这种引力下的演化行为。我们还利用扰动技术进行了稳定性分析。我们的研究结果表明,在反弹点处违反了空能条件,状态方程参数表现出五元时代或幻影状态的特征。这些方面凸显了反弹宇宙学模型中能量条件与稳定性之间复杂的相互作用。我们的结论是:(f(mathcal {R},T^2)) 理论成功地为标准宇宙学方案提供了可行的替代方案,为早期宇宙和引力的本质提供了见解。
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引用次数: 0
Hidden attractors in fractional-order discrete maps 分数阶离散映射中的隐藏吸引子
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2024-10-21 DOI: 10.1140/epjb/s10051-024-00780-7
Vaibhav Varshney, S. Leo Kingston, Sabarathinam Srinivasan, Suresh Kumarasamy

This study investigates the hidden dynamics of fractional-order discrete two-dimensional maps, focusing on the generation of hidden attractors and the impact of order on their size and boundaries. Three different nonlinear maps are used, and various measures, such as phase portraits, bifurcation diagrams, and basin of attraction, are presented. This study also observes changes in basin boundaries of hidden attractors with varying order. The rational memristive maps exhibit a well-defined basin of attraction for a broad range of system orders, with multistability and a riddled basin for some orders. The memristive Gauss map also shows well-defined and riddled basins, however, the quadratic chaotic map demonstrates a decreasing basin size and a riddled basin boundary for higher orders of the system.

本研究探讨了分数阶离散二维地图的隐藏动力学,重点是隐藏吸引子的产生以及阶数对其大小和边界的影响。本研究使用了三种不同的非线性映射,并给出了各种测量方法,如相肖像、分岔图和吸引盆。这项研究还观察了不同阶数下隐藏吸引子盆地边界的变化。在广泛的系统阶数范围内,有理忆阻图表现出定义明确的吸引盆地,在某些阶数上具有多稳定性,并呈现出千疮百孔的盆地。忆阻性高斯图也显示出定义明确的海盆和千疮百孔的海盆,然而,二次混沌图则显示出海盆大小不断减小,且系统阶数越高,海盆边界越千疮百孔。
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引用次数: 0
Vuv/vis absorption spectroscopy of different PAHs 不同多环芳烃的 Vuv/vis 吸收光谱分析
IF 2.5 4区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-21 DOI: 10.1007/s00339-024-07959-w
Lorenzo Maddii Fabiani, Tobias Reiker, Helmut Zacharias

The present study provides new solid-phase absorption data of different Polycyclic Aromatic Hydrocarbon (PAHs) molecules in the Far Ultraviolet (FUV) and UV/Visible regions. Two features of interstellar extinction curves fall in this region: the FUV rise and the UV bump. Here, thin films of PAHs were prepared by means of the spin coating method onto a transparent substrate, and their solid phase absorption spectra were recorded. Spectra of isolated molecules simulated by Time-Dependent Density Functional Theory (TD-DFT) calculations were also produced for comparison. The results fit quite well with the FUV rise but not with the UV bump. Given the scarcity of FUV experimental absorption data of PAHs in the literature and especially in solid phase, these results are also interesting for reference for other studies ranging from thin films applications to interstellar medium models.

本研究提供了不同多环芳香烃(PAHs)分子在远紫外(FUV)和紫外/可见光区域的新固相吸收数据。星际消光曲线的两个特征位于该区域:FUV 上升和紫外凹凸。在此,我们采用旋涂法在透明基底上制备了多环芳烃薄膜,并记录了它们的固相吸收光谱。为了进行比较,还利用时变密度泛函理论(TD-DFT)计算模拟了分离分子的光谱。结果与紫外波段的上升相当吻合,但与紫外波段的凸起不吻合。鉴于多环芳烃的 FUV 实验吸收数据在文献中,特别是在固相中非常稀少,这些结果对于从薄膜应用到星际介质模型的其他研究也有参考价值。
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引用次数: 0
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