Pub Date : 2026-11-01Epub Date: 2026-08-31DOI: 10.1177/15311074261483400
Alexander Engel, Henry Strasdeit, Stefan Fox, Ronny Löffler
Chemical biosignatures, if present, are exposed to ultraviolet (UV) radiation at several locations in the solar system, including the martian surface. Solid thin-layer samples are commonly used to study the effect of UV irradiation on the stability of potential organic biosignatures in the laboratory and in space. Given the limitations of the layer deposition techniques previously used in astrobiology experiments, such as sublimation-recondensation and casting, antisolvent precipitation (i.e., crystallization from solution by addition of a poor solvent) offers a promising alternative. We applied the latter technique to deposit optically opaque crystalline layers of 1-methylnicotinamide chloride ((MNA)Cl) for use in subsequent UV irradiation experiments. The 1-methylnicotinamide cation in (MNA)Cl serves as a model of hypothetical extraterrestrial nicotinamide-based redox cofactors related to NAD(P)+. Under UV irradiation (λ ≥ 224 nm), decomposition of (MNA)Cl occurred, but it ceased after ∼14 days, leaving a large fraction of the material intact. This behavior is attributed to the shielding effect of a photoproduct layer on the crystal surfaces and can be kinetically described by a first-order bounded decay model. Such "self-preservation" may enhance the survivability of certain organic biosignatures provided they form sufficiently thick (opaque) layers or crystals. The presence of either synthetic gypsum (CaSO4·2H2O) or halite (NaCl) had a minimal effect on the kinetic parameters of the UV decomposition of (MNA)Cl.
{"title":"UV Exposure Study of 1-Methylnicotinamide Chloride: Self-Preservation in a Simple NAD(P)<sup>+</sup> Analog.","authors":"Alexander Engel, Henry Strasdeit, Stefan Fox, Ronny Löffler","doi":"10.1177/15311074261483400","DOIUrl":"10.1177/15311074261483400","url":null,"abstract":"<p><p>Chemical biosignatures, if present, are exposed to ultraviolet (UV) radiation at several locations in the solar system, including the martian surface. Solid thin-layer samples are commonly used to study the effect of UV irradiation on the stability of potential organic biosignatures in the laboratory and in space. Given the limitations of the layer deposition techniques previously used in astrobiology experiments, such as sublimation-recondensation and casting, antisolvent precipitation (<i>i.e.</i>, crystallization from solution by addition of a poor solvent) offers a promising alternative. We applied the latter technique to deposit optically opaque crystalline layers of 1-methylnicotinamide chloride ((MNA)Cl) for use in subsequent UV irradiation experiments. The 1-methylnicotinamide cation in (MNA)Cl serves as a model of hypothetical extraterrestrial nicotinamide-based redox cofactors related to NAD(P)<sup>+</sup>. Under UV irradiation (<i>λ</i> ≥ 224 nm), decomposition of (MNA)Cl occurred, but it ceased after ∼14 days, leaving a large fraction of the material intact. This behavior is attributed to the shielding effect of a photoproduct layer on the crystal surfaces and can be kinetically described by a first-order bounded decay model. Such \"self-preservation\" may enhance the survivability of certain organic biosignatures provided they form sufficiently thick (opaque) layers or crystals. The presence of either synthetic gypsum (CaSO<sub>4</sub>·2H<sub>2</sub>O) or halite (NaCl) had a minimal effect on the kinetic parameters of the UV decomposition of (MNA)Cl.</p>","PeriodicalId":8645,"journal":{"name":"Astrobiology","volume":" ","pages":"950-966"},"PeriodicalIF":2.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148863504","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The transition to sustained human space exploration is reshaping how astrobiology can be conducted. As missions extend beyond low Earth orbit and involve governmental and commercial actors, astrobiology is increasingly becoming embedded in complex operational and policy environments. These developments can be seen as a shift in the operational, interpretive, and governance contexts of astrobiology, affecting how investigations are conducted, how findings are interpreted, and how research is coordinated across mission phases. Here, we outline the implications of human presence for astrobiology research and its integration within evolving exploration architectures, and examine its role in future missions.
{"title":"The Case for Integrating Astrobiology Before, During, and After Crewed Space Missions.","authors":"Celia Blanco, Anamaria Berea, Anurup Mohanty, Arunava Poddar, Rajat Bhushan Gupta","doi":"10.1177/15311074261484862","DOIUrl":"10.1177/15311074261484862","url":null,"abstract":"<p><p>The transition to sustained human space exploration is reshaping how astrobiology can be conducted. As missions extend beyond low Earth orbit and involve governmental and commercial actors, astrobiology is increasingly becoming embedded in complex operational and policy environments. These developments can be seen as a shift in the operational, interpretive, and governance contexts of astrobiology, affecting how investigations are conducted, how findings are interpreted, and how research is coordinated across mission phases. Here, we outline the implications of human presence for astrobiology research and its integration within evolving exploration architectures, and examine its role in future missions.</p>","PeriodicalId":8645,"journal":{"name":"Astrobiology","volume":" ","pages":"944-949"},"PeriodicalIF":2.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148904946","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-11-01Epub Date: 2026-08-31DOI: 10.1177/15311074261483387
Rui-Lin Cheng, Carolina Munoz-Saez, Kathleen A Campbell, Joseph R Michalski, Andrew D Czaja, Steven W Ruff
Silica sinters are promising astrobiology targets in the search for signs of past extraterrestrial life on Mars. Although terrestrial sinter morphologic features may serve as potential biosignatures at the macroscale, identification of carbonaceous matter (CM) within silica would offer substantial support for interpreting martian silica deposits as having a biologic association. Raman spectroscopy provides a means to identify both minerals and organics in situ. This technique has been employed to analyze CM in terrestrial sinters that consist of microcrystalline quartz and has also been deployed previously on Mars to search for organics. However, martian silica deposits are dominated by opaline silica rather than quartz, and a thorough examination of CM within terrestrial opaline silica by Raman spectroscopy is generally lacking. We investigated opaline silica sinters from northern Chile, an exceptional terrestrial analog for Mars, by Raman spectroscopy with multiple excitations. Our results show that strong fluorescence from opaline silica modifies CM Raman spectral signatures across excitation wavelengths. CM Raman spectra within opaline silica sinters vary both among facies and within individual samples, and they differ from those in Archean cherts. This study demonstrates that reliable interpretation of CM Raman spectra requires attention to host-matrix influences, excitation wavelength, and curve-fitting procedures.
{"title":"Multi-Excitation Raman Spectroscopy of Carbonaceous Matter within Opaline Silica Sinters from Mars-Analog Hot Spring Settings: Implications for the Search for Extraterrestrial Biosignatures.","authors":"Rui-Lin Cheng, Carolina Munoz-Saez, Kathleen A Campbell, Joseph R Michalski, Andrew D Czaja, Steven W Ruff","doi":"10.1177/15311074261483387","DOIUrl":"10.1177/15311074261483387","url":null,"abstract":"<p><p>Silica sinters are promising astrobiology targets in the search for signs of past extraterrestrial life on Mars. Although terrestrial sinter morphologic features may serve as potential biosignatures at the macroscale, identification of carbonaceous matter (CM) within silica would offer substantial support for interpreting martian silica deposits as having a biologic association. Raman spectroscopy provides a means to identify both minerals and organics <i>in situ</i>. This technique has been employed to analyze CM in terrestrial sinters that consist of microcrystalline quartz and has also been deployed previously on Mars to search for organics. However, martian silica deposits are dominated by opaline silica rather than quartz, and a thorough examination of CM within terrestrial opaline silica by Raman spectroscopy is generally lacking. We investigated opaline silica sinters from northern Chile, an exceptional terrestrial analog for Mars, by Raman spectroscopy with multiple excitations. Our results show that strong fluorescence from opaline silica modifies CM Raman spectral signatures across excitation wavelengths. CM Raman spectra within opaline silica sinters vary both among facies and within individual samples, and they differ from those in Archean cherts. This study demonstrates that reliable interpretation of CM Raman spectra requires attention to host-matrix influences, excitation wavelength, and curve-fitting procedures.</p>","PeriodicalId":8645,"journal":{"name":"Astrobiology","volume":" ","pages":"967-983"},"PeriodicalIF":2.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148863557","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-11-01Epub Date: 2026-08-31DOI: 10.1177/15311074261483886
Arsev Umur Aydinoglu, Ozgur Kadir Ozer
This study presents an analysis of diversity, equity, and inclusion in the U.S. astrobiology community. Using national survey data, we examined how gender, race, age, and career stage affect researchers' experiences with mentorship, funding, and career advancement. The results reveal disparities: female participants reported gender discrimination at seven times the rate of male respondents, and 85% of all respondents had encountered harassment. Nearly half experienced career interruptions, most commonly due to mental health challenges (57%), family obligations, or harassment. Other persistent barriers included difficulty meeting workplace expectations (84%), securing permanent positions (40%), and obtaining adequate funding (nearly one-third). Female researchers reported lower levels of workplace support and collegial respect than their male peers. While some institutions have begun implementing equity-focused practices, adoption across the field remains limited. Based on these findings, we recommend that institutions publicly report diversity metrics, establish targeted mentorship programs, and provide mental health support and parental leave policies. Addressing these systemic barriers is essential not only for ethical reasons but also for advancing astrobiology's mission, which depends on diverse perspectives and collaboration.
{"title":"Diversity Lost in Space: Discrimination and Exclusion in Astrobiology.","authors":"Arsev Umur Aydinoglu, Ozgur Kadir Ozer","doi":"10.1177/15311074261483886","DOIUrl":"10.1177/15311074261483886","url":null,"abstract":"<p><p>This study presents an analysis of diversity, equity, and inclusion in the U.S. astrobiology community. Using national survey data, we examined how gender, race, age, and career stage affect researchers' experiences with mentorship, funding, and career advancement. The results reveal disparities: female participants reported gender discrimination at seven times the rate of male respondents, and 85% of all respondents had encountered harassment. Nearly half experienced career interruptions, most commonly due to mental health challenges (57%), family obligations, or harassment. Other persistent barriers included difficulty meeting workplace expectations (84%), securing permanent positions (40%), and obtaining adequate funding (nearly one-third). Female researchers reported lower levels of workplace support and collegial respect than their male peers. While some institutions have begun implementing equity-focused practices, adoption across the field remains limited. Based on these findings, we recommend that institutions publicly report diversity metrics, establish targeted mentorship programs, and provide mental health support and parental leave policies. Addressing these systemic barriers is essential not only for ethical reasons but also for advancing astrobiology's mission, which depends on diverse perspectives and collaboration.</p>","PeriodicalId":8645,"journal":{"name":"Astrobiology","volume":" ","pages":"984-997"},"PeriodicalIF":2.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148863514","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-11-01Epub Date: 2026-09-15DOI: 10.1177/15311074261484864
Alfonso Davila, Tori Hoehler, Svetlana Shkolyar, Michel Nuevo, Karyn Rogers, Laura M Barge, Alexis Bouquet, Jacob Buffo, Aaron Burton, Morgan Cable, H James Cleaves, Andrew D Czaja, Grégoire Danger, Moran Frenkel-Pinter, Christopher German, Stephanie Getty, Christopher Glein, Heather Graham, Kevin Hand, Sarah Hörst, Kristin Johnson-Finn, Wanying Kang, Ramanarayanan Krishnamurthy, Shannon MacKenzie, Aaron Noell, Frank Postberg, Andro Rios, Jeffrey Seewald, Barbara Sherwood Lollar, Andrew Steele, Ichiko Sugiyama
The "Exploring the Abiotic Background for Life Detection" workshop was convened between March 31, 2025, and April 3, 2025, at the Carnegie Institution for Science in Washington, D.C. The workshop gathered scientists and technologists from different disciplines and career stages to consider the "abiotic background": recognizing, characterizing, and understanding the set of abiotic substances, structures, and processes that may result in potential false-positive or false-negative results in the search for evidence of life beyond Earth. To frame the conversation and ensure programmatic relevance, the workshop emphasized Ocean Worlds, while also leveraging lessons learned from modern and early Earth and Mars. Salient takeaways include the following: (1) a large abiotic background, potentially sustained over geologic timescales, could mimic, obscure, and alter biosignatures, posing risks of false positives and false negatives. Addressing these challenges requires balancing targeted and untargeted measurements within the constraints of robotic spacecraft payloads; (2) the search for signatures of life beyond Earth represents a sharp inflection point in spacecraft mission complexity and design. Stakeholders of such missions must strike a difficult balance between scientific aspirations and the technological constraints inherent to robotic spaceflight; (3) Ocean Worlds are a distinct class of habitable environments, each with unique evolutionary pathways, but collectively offering new opportunities to study organic chemical evolution; (4) there is a need to establish community-wide experimental standards and laboratory simulations to better constrain the range of abiotic chemistry and improve abiotic chemistry models to guide the design of spacecraft missions; (5) a unifying, predictive framework for abiotic chemical evolution could provide a robust baseline for interpreting mission data and guiding future exploration. This report seeks to catalyze a sustained and focused dialogue on how to best account for the abiotic background in the design of astrobiology spacecraft missions. By framing the issue both in terms of risks and scientific opportunities, we lay the groundwork for a richer, more integrated approach to the exploration of other worlds that benefits from continued cross-disciplinary input. We contend that advancing our understanding of the abiotic background now will directly inform and improve future astrobiological spacecraft missions, particularly in terms of payload selection and data interpretation.
{"title":"The Abiotic Background: Challenges and Opportunities in the Search for Evidence of Life Beyond Earth.","authors":"Alfonso Davila, Tori Hoehler, Svetlana Shkolyar, Michel Nuevo, Karyn Rogers, Laura M Barge, Alexis Bouquet, Jacob Buffo, Aaron Burton, Morgan Cable, H James Cleaves, Andrew D Czaja, Grégoire Danger, Moran Frenkel-Pinter, Christopher German, Stephanie Getty, Christopher Glein, Heather Graham, Kevin Hand, Sarah Hörst, Kristin Johnson-Finn, Wanying Kang, Ramanarayanan Krishnamurthy, Shannon MacKenzie, Aaron Noell, Frank Postberg, Andro Rios, Jeffrey Seewald, Barbara Sherwood Lollar, Andrew Steele, Ichiko Sugiyama","doi":"10.1177/15311074261484864","DOIUrl":"10.1177/15311074261484864","url":null,"abstract":"<p><p>The \"Exploring the Abiotic Background for Life Detection\" workshop was convened between March 31, 2025, and April 3, 2025, at the Carnegie Institution for Science in Washington, D.C. The workshop gathered scientists and technologists from different disciplines and career stages to consider the \"abiotic background\": recognizing, characterizing, and understanding the set of abiotic substances, structures, and processes that may result in potential false-positive or false-negative results in the search for evidence of life beyond Earth. To frame the conversation and ensure programmatic relevance, the workshop emphasized Ocean Worlds, while also leveraging lessons learned from modern and early Earth and Mars. Salient takeaways include the following: (1) a large abiotic background, potentially sustained over geologic timescales, could mimic, obscure, and alter biosignatures, posing risks of false positives and false negatives. Addressing these challenges requires balancing targeted and untargeted measurements within the constraints of robotic spacecraft payloads; (2) the search for signatures of life beyond Earth represents a sharp inflection point in spacecraft mission complexity and design. Stakeholders of such missions must strike a difficult balance between scientific aspirations and the technological constraints inherent to robotic spaceflight; (3) Ocean Worlds are a distinct class of habitable environments, each with unique evolutionary pathways, but collectively offering new opportunities to study organic chemical evolution; (4) there is a need to establish community-wide experimental standards and laboratory simulations to better constrain the range of abiotic chemistry and improve abiotic chemistry models to guide the design of spacecraft missions; (5) a unifying, predictive framework for abiotic chemical evolution could provide a robust baseline for interpreting mission data and guiding future exploration. This report seeks to catalyze a sustained and focused dialogue on how to best account for the abiotic background in the design of astrobiology spacecraft missions. By framing the issue both in terms of risks and scientific opportunities, we lay the groundwork for a richer, more integrated approach to the exploration of other worlds that benefits from continued cross-disciplinary input. We contend that advancing our understanding of the abiotic background now will directly inform and improve future astrobiological spacecraft missions, particularly in terms of payload selection and data interpretation.</p>","PeriodicalId":8645,"journal":{"name":"Astrobiology","volume":" ","pages":"927-943"},"PeriodicalIF":2.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148966325","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Solar‐blind polarization photodetectors are highly desirable for next‐generation intelligent sensing and imaging systems, yet achieving a high polarization ratio remains a major challenge for current devices. Here, we report a solar‐blind polarization photodetector based on mechanically exfoliated β ‐Ga 2 O 3 microwires, in which intrinsic crystal anisotropy and morphology‐induced anisotropy are synergistically combined to enable enhanced polarization‐sensitive photoresponse. First‐principles calculations reveal that the intrinsic anisotropic optical absorption of β ‐Ga 2 O 3 originates from its low‐symmetry monoclinic crystal structure, leading to polarization‐dependent interband transitions. The finite‐difference time‐domain (FDTD) simulations reveal that the microwire morphology introduces additional polarization‐dependent optical anisotropy. A simple metal‐semiconductor‐metal photodetector is constructed using a single β ‐Ga 2 O 3 microwire, achieving outstanding solar‐blind ultraviolet detection performance with an ultrahigh polarization ratio (PR) of 5200. Furthermore, by integrating the anisotropic photoresponse into a polarization convolution (pCONV) and combining it with an artificial neural network, high‐accuracy fingerprint recognition is achieved with an accuracy of about 99%. This work establishes β ‐Ga 2 O 3 microwires as a promising material for high‐performance solar‐blind polarization photodetection and highlights the effectiveness of morphology engineering in boosting polarization‐sensitive optoelectronic performance.
{"title":"Solar‐Blind Polarization Sensitive Photodetection Based on β‐ Ga 2 O 3 Microwires With Super‐High Polarization Ratio (>5000) Enabled by Intrinsic and Morphological Anisotropy","authors":"Xiaoyu Jiang, Yiwen Zhang, Zhihao Yu, Yiding Jian, Chao Wu, Hao Wu, Shunli Wang, Daoyou Guo","doi":"10.1002/lpor.72152","DOIUrl":"https://doi.org/10.1002/lpor.72152","url":null,"abstract":"Solar‐blind polarization photodetectors are highly desirable for next‐generation intelligent sensing and imaging systems, yet achieving a high polarization ratio remains a major challenge for current devices. Here, we report a solar‐blind polarization photodetector based on mechanically exfoliated <jats:italic>β</jats:italic> ‐Ga <jats:sub>2</jats:sub> O <jats:sub>3</jats:sub> microwires, in which intrinsic crystal anisotropy and morphology‐induced anisotropy are synergistically combined to enable enhanced polarization‐sensitive photoresponse. First‐principles calculations reveal that the intrinsic anisotropic optical absorption of <jats:italic>β</jats:italic> ‐Ga <jats:sub>2</jats:sub> O <jats:sub>3</jats:sub> originates from its low‐symmetry monoclinic crystal structure, leading to polarization‐dependent interband transitions. The finite‐difference time‐domain (FDTD) simulations reveal that the microwire morphology introduces additional polarization‐dependent optical anisotropy. A simple metal‐semiconductor‐metal photodetector is constructed using a single <jats:italic>β</jats:italic> ‐Ga <jats:sub>2</jats:sub> O <jats:sub>3</jats:sub> microwire, achieving outstanding solar‐blind ultraviolet detection performance with an ultrahigh polarization ratio (PR) of 5200. Furthermore, by integrating the anisotropic photoresponse into a polarization convolution (pCONV) and combining it with an artificial neural network, high‐accuracy fingerprint recognition is achieved with an accuracy of about 99%. This work establishes <jats:italic>β</jats:italic> ‐Ga <jats:sub>2</jats:sub> O <jats:sub>3</jats:sub> microwires as a promising material for high‐performance solar‐blind polarization photodetection and highlights the effectiveness of morphology engineering in boosting polarization‐sensitive optoelectronic performance.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"84 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2026-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149292699","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Upconverting quantum dots (UCQDs) represent a class of emerging semiconductor nanocrystals that can convert long‐wavelength excitation photons into higher‐energy visible or ultraviolet emissions via an anti‐Stokes process, thereby overcoming the reliance of conventional quantum dots on short‐wavelength excitations. Owning to their unique physicochemical properties such as deeper tissue penetration, reduced photodamage, high signal‐to‐noise ratio and more efficient use of near infrared (NIR) photons, UCQDs are broadly applied in bioimaging, phototherapy, photodetection, solar cell, etc. This review firstly introduces the advantages of long‐wavelength excitable luminescence and the superior optical properties of UCQDs compared to their counterparts. It then summarizes state‐of‐the‐art approaches to construct UCQDs. Specifically, intrinsic mechanisms based on multiphoton absorption, phonon‐assisted upconversion and exciton interactions in quantum‐dot heterostructures are discussed. Hybrid systems are also covered, in which quantum dots act as sensitizers for triplet–triplet annihilation or couple with lanthanide‐doped upconversion nanoparticles. Subsequently, emerging applications of UCQDs in in vivo imaging, phototherapy, photodetection and solar cells are presented. Finally, current challenges and future perspectives for the development of UCQDs are provided as a conclusion.
{"title":"Exploring Photon‐Upconverting Quantum Dots: From Strategic Design to Diverse Applications","authors":"Huadong Chen, Haomin Chen, Ming Tang, Jing Wang, Wenqian Chen, Xiaohui Zhu, Yong Zhang","doi":"10.1002/lpor.72151","DOIUrl":"https://doi.org/10.1002/lpor.72151","url":null,"abstract":"Upconverting quantum dots (UCQDs) represent a class of emerging semiconductor nanocrystals that can convert long‐wavelength excitation photons into higher‐energy visible or ultraviolet emissions via an anti‐Stokes process, thereby overcoming the reliance of conventional quantum dots on short‐wavelength excitations. Owning to their unique physicochemical properties such as deeper tissue penetration, reduced photodamage, high signal‐to‐noise ratio and more efficient use of near infrared (NIR) photons, UCQDs are broadly applied in bioimaging, phototherapy, photodetection, solar cell, etc. This review firstly introduces the advantages of long‐wavelength excitable luminescence and the superior optical properties of UCQDs compared to their counterparts. It then summarizes state‐of‐the‐art approaches to construct UCQDs. Specifically, intrinsic mechanisms based on multiphoton absorption, phonon‐assisted upconversion and exciton interactions in quantum‐dot heterostructures are discussed. Hybrid systems are also covered, in which quantum dots act as sensitizers for triplet–triplet annihilation or couple with lanthanide‐doped upconversion nanoparticles. Subsequently, emerging applications of UCQDs in in vivo imaging, phototherapy, photodetection and solar cells are presented. Finally, current challenges and future perspectives for the development of UCQDs are provided as a conclusion.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"17 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2026-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149292701","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Fan Yang, Zhen Liu, Yang‐Hui Huang, Ma‐Lin Zhong, Jie Deng, Yu Nie, Nai‐Tao Liu, Sai‐Ying Ru, Zhen‐Guo Li, Long Wang, Yao‐Yao Pan, Chang‐Wei Sun, Xue‐Cou Tu, La‐Bao Zhang, Xiao‐Qing Jia, Lin Kang, Qing‐Yuan Zhao, Jian Chen, Pei‐Heng Wu
Although photodetector integration on waveguides is advanced, optical fiber lacks advantages in integration scalability. Integrating multiple photodetectors enables multi‐dimensional photon information acquisition, which is crucial for quantum information science. Here, fiber‐integrated dual‐layer SNSPDs with orthogonal polarization sensitivity and coincidence detection capability are demonstrated. Two SNSPD membranes were sequentially transferred onto a fiber facet with orthogonal nanowire orientations. At 1550 nm, the top and bottom layers exhibited system detection efficiency (SDE) of 49.6% and 42.4%, and polarization extinction ratio (PER), which is defined as the ratio of the maximum to minimum SDE, of 3.94 and 4.37, respectively. Summing the two signals increased the system detection efficiency to 57.9%–60.7% and reduced the overall PER to 1.06–1.14 across 1480–1640 nm. By reading each layer individually, coincidence measurement can be performed directly within the fiber with an overall timing jitter of 86 ps, characterized by femtosecond laser pulses. This work demonstrates multi‐dimensional single‐photon detection and the potential for fiber‐integrated quantum circuits.
{"title":"Fiber‐Integrated Stacking Superconducting Nanowire Single‐Photon Detectors With Orthogonal Polarization Sensitivity and Coincidence Detection","authors":"Fan Yang, Zhen Liu, Yang‐Hui Huang, Ma‐Lin Zhong, Jie Deng, Yu Nie, Nai‐Tao Liu, Sai‐Ying Ru, Zhen‐Guo Li, Long Wang, Yao‐Yao Pan, Chang‐Wei Sun, Xue‐Cou Tu, La‐Bao Zhang, Xiao‐Qing Jia, Lin Kang, Qing‐Yuan Zhao, Jian Chen, Pei‐Heng Wu","doi":"10.1002/lpor.72137","DOIUrl":"https://doi.org/10.1002/lpor.72137","url":null,"abstract":"Although photodetector integration on waveguides is advanced, optical fiber lacks advantages in integration scalability. Integrating multiple photodetectors enables multi‐dimensional photon information acquisition, which is crucial for quantum information science. Here, fiber‐integrated dual‐layer SNSPDs with orthogonal polarization sensitivity and coincidence detection capability are demonstrated. Two SNSPD membranes were sequentially transferred onto a fiber facet with orthogonal nanowire orientations. At 1550 nm, the top and bottom layers exhibited system detection efficiency (SDE) of 49.6% and 42.4%, and polarization extinction ratio (PER), which is defined as the ratio of the maximum to minimum SDE, of 3.94 and 4.37, respectively. Summing the two signals increased the system detection efficiency to 57.9%–60.7% and reduced the overall PER to 1.06–1.14 across 1480–1640 nm. By reading each layer individually, coincidence measurement can be performed directly within the fiber with an overall timing jitter of 86 ps, characterized by femtosecond laser pulses. This work demonstrates multi‐dimensional single‐photon detection and the potential for fiber‐integrated quantum circuits.","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"5 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2026-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149292702","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Correction to “High Spatial and Angular Resolution Wavefront Sensing Based on the Random Phase Modulated Diffraction Effect”","authors":"","doi":"10.1002/lpor.72158","DOIUrl":"https://doi.org/10.1002/lpor.72158","url":null,"abstract":"","PeriodicalId":204,"journal":{"name":"Laser & Photonics Reviews","volume":"4 1","pages":""},"PeriodicalIF":11.0,"publicationDate":"2026-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149292698","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2026-10-30DOI: 10.22331/q-2026-10-30-2257
Benjamin Yadin, Matteo Fadel
The notion of a macroscopic quantum state must be pinned down in order to assess how well experiments probe the large-scale limits of quantum mechanics. However, the issue of quantifying so-called quantum macroscopicity is fraught with multiple approaches having varying interpretations and levels of computability and measurability. Here, we introduce two measures that capture independent macroscopic properties: i) extensive size, measuring the degree of coherence in position or momentum observables relative to atomic-scale units, and ii) entangled size, quantifying the number of entangled subsystems. These measures unify many desirable features of past proposals while having rigorously justified interpretations from quantum information theory in terms of coherence and multipartite entanglement. We demonstrate how to estimate them and obtain lower-bounds using experimental data from micro-mechanical oscillators and diffracting molecules. Notably, we find evidence for genuine multipartite entanglement of $10^5$ to $10^7$ atoms in recent mechanical superposition states.
{"title":"Macroscopic quantum coherence and entanglement in mechanical systems","authors":"Benjamin Yadin, Matteo Fadel","doi":"10.22331/q-2026-10-30-2257","DOIUrl":"https://doi.org/10.22331/q-2026-10-30-2257","url":null,"abstract":"The notion of a macroscopic quantum state must be pinned down in order to assess how well experiments probe the large-scale limits of quantum mechanics. However, the issue of quantifying so-called quantum macroscopicity is fraught with multiple approaches having varying interpretations and levels of computability and measurability. Here, we introduce two measures that capture independent macroscopic properties: i) extensive size, measuring the degree of coherence in position or momentum observables relative to atomic-scale units, and ii) entangled size, quantifying the number of entangled subsystems. These measures unify many desirable features of past proposals while having rigorously justified interpretations from quantum information theory in terms of coherence and multipartite entanglement. We demonstrate how to estimate them and obtain lower-bounds using experimental data from micro-mechanical oscillators and diffracting molecules. Notably, we find evidence for genuine multipartite entanglement of $10^5$ to $10^7$ atoms in recent mechanical superposition states.","PeriodicalId":20807,"journal":{"name":"Quantum","volume":"9 1","pages":""},"PeriodicalIF":6.4,"publicationDate":"2026-10-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149287878","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}