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Class-Selective Spin Activity of Two Spectrally Distinct Color Centers in Oxygen-Annealed Hexagonal Boron Nitride
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-11-02 DOI: 10.1021/acsphotonics.6c01777
Yuxing Liu,Pankaj Kumar,Abhishek Trivedi,Moksh Khatri,Eui-Hyeok Yang,Stefan Strauf
Hexagonal boron nitride (hBN) hosts a variety of room-temperature single-photon emitters, among which optically addressable spin defects are attractive for quantum sensing and spin–photon interfaces. While the negatively charged boron vacancy is well established as an ensemble spin system, bright and individually addressable spin-active emitters remain scarce, and it is unknown whether spin activity is a property of an entire optical emitter class or only of a subset. We have recently shown that oxygen annealing of hBN activates two spectrally distinct emitter populations with so-far unresolved spin properties. Here, we perform optically detected magnetic resonance (ODMR) screening of 158 individual emitters across both populations. We find that spin activity is carried exclusively by the Type I population: 9 of 100 Type I emitters display ODMR with coexisting S = 1 and S = 1/2 transitions and zero-field splitting (ZFS) parameters of D ≈ 977 MHz and E ≈ 174 MHz, while all 58 Type II emitters remain spin-silent. Pulsed ODMR on all three transition branches reveals spin–lattice relaxation times up to 19.1 μs and spin echo coherence times up to 56.0 ns, with the S = 1/2 branch showing systematically shorter T2 than the two S = 1 branches in every spin-active emitter. The exclusive correlation of spin activity with one optical class and the branch-resolved coherence asymmetry provide experimental constraints for identifying the microscopic origin of carbon- and oxygen-related color centers in hBN.
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引用次数: 0
Design of Monolithic Microcavities for Enhancing Organic Quantum Emitters
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-11-02 DOI: 10.1021/acsphotonics.6c02097
Tim Hebenstreit,Jaime Gimeno Balaguer,Fridtjof Betz,Felix Binkowski,Maja Colautti,Jan Renger,Costanza Toninelli,Sven Burger,Stephan Götzinger
Single organic molecules are a well-established platform for high-quality single-photon generation: they can emit lifetime-limited photons with high purity and indistinguishability. However, their emission is accompanied by a pronounced red-shifted phonon sideband and higher-order vibrational peaks, which reduce the fraction of photons emitted into the desired narrowband zero-phonon line. The standard approach to suppressing this unwanted emission is to integrate the emitter into a monolithic photonic nanostructure that provides Purcell enhancement. However, incorporating organic materials using clean-room techniques has proven challenging and has, in fact, so far prevented the integration of single molecules in crystalline hosts into monolithic microcavities. As a result, efficient, narrowband organic single-photon sources for applications in quantum information processing have remained elusive despite their considerable promise. Here, we propose three monolithic microcavity designs tailored to provide sufficient Purcell enhancement for organic quantum emitters. The Purcell effect induced by these cavities preferentially enhances emission into the 0–0 zero-phonon line, increasing spectral purity, photon extraction, and shortening the excited-state lifetime, which in turn relaxes the requirements for generating indistinguishable photons. The cavities have been optimized using Bayesian optimization and the adaptive Antoulas–Anderson (AAA) algorithm for rational approximation, which offer global optimization and the efficient reconstruction of spectra from scattering simulations, respectively. These structures are compatible with both standard clean-room processing and single-molecule preparation techniques. Therefore, they offer a clear route to realizing high-quality, practically monochromatic organic single-photon light sources.
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引用次数: 0
Monolithically Integrated Active-Cavity “Laser-as-a-Sensor”: Active Intracavity Enhancement for Oxygen Detection with a Subnanoliter Sampling Volume
IF 7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-11-02 DOI: 10.1021/acsphotonics.6c02294
Hongzhuo Wang,Lichao Zhang,Ning Cui,Jisheng Wang,Jingyu Liu,Baolu Guan
Tunable diode laser absorption spectroscopy (TDLAS) is widely used in O2 gas sensing; however, conventional schemes rely on meter-scale optical path lengths and hundred-milliliter absorption cells, making it difficult to meet the demands of chip-scale integration and distributed sensing. This paper proposes and demonstrates a 760 nm microelectromechanical (MEMS) vertical-cavity surface-emitting laser (VCSEL) gas sensor with a monolithically integrated active cavity. The active cavity and the sensing function are monolithically integrated; the active cavity simultaneously serves as the gas absorption cell, integrating wavelength tuning, gain compensation, and gas absorption into the same active microcavity. Continuous single-mode tuning is achieved in the 760–764 nm range (side-mode suppression ratio >30 dB). The intracavity amplified absorption (IAA) effect enables a sampling volume of only subnanoliter, which is 7–8 orders of magnitude smaller than conventional hundred-milliliter gas cells. Based on the nonlinear modulation response of threshold output power to intracavity absorption, an equivalent optical path enhancement factor of 1.3 × 105 is achieved, with a limit of detection reaching 37 ppm. This “laser-as-a-sensor” architecture offers a compact route for chip-scale distributed gas sensing networks.
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引用次数: 0
UV Exposure Study of 1-Methylnicotinamide Chloride: Self-Preservation in a Simple NAD(P)+ Analog. 1-甲基烟酰胺氯的紫外暴露研究:在简单NAD(P)+类似物中的自我保存。
IF 2.3 3区 物理与天体物理 Q2 ASTRONOMY & ASTROPHYSICS Pub Date : 2026-11-01 Epub Date: 2026-08-31 DOI: 10.1177/15311074261483400
Alexander Engel, Henry Strasdeit, Stefan Fox, Ronny Löffler

Chemical biosignatures, if present, are exposed to ultraviolet (UV) radiation at several locations in the solar system, including the martian surface. Solid thin-layer samples are commonly used to study the effect of UV irradiation on the stability of potential organic biosignatures in the laboratory and in space. Given the limitations of the layer deposition techniques previously used in astrobiology experiments, such as sublimation-recondensation and casting, antisolvent precipitation (i.e., crystallization from solution by addition of a poor solvent) offers a promising alternative. We applied the latter technique to deposit optically opaque crystalline layers of 1-methylnicotinamide chloride ((MNA)Cl) for use in subsequent UV irradiation experiments. The 1-methylnicotinamide cation in (MNA)Cl serves as a model of hypothetical extraterrestrial nicotinamide-based redox cofactors related to NAD(P)+. Under UV irradiation (λ ≥ 224 nm), decomposition of (MNA)Cl occurred, but it ceased after ∼14 days, leaving a large fraction of the material intact. This behavior is attributed to the shielding effect of a photoproduct layer on the crystal surfaces and can be kinetically described by a first-order bounded decay model. Such "self-preservation" may enhance the survivability of certain organic biosignatures provided they form sufficiently thick (opaque) layers or crystals. The presence of either synthetic gypsum (CaSO4·2H2O) or halite (NaCl) had a minimal effect on the kinetic parameters of the UV decomposition of (MNA)Cl.

化学生物特征,如果存在的话,在太阳系的几个地方暴露在紫外线(UV)辐射下,包括火星表面。固体薄层样品通常用于研究紫外线照射对实验室和太空中潜在有机生物特征稳定性的影响。考虑到先前在天体生物学实验中使用的层沉积技术的局限性,例如升华-再冷凝和铸造,反溶剂沉淀法(即通过添加弱溶剂从溶液中结晶)提供了一个有希望的替代方法。我们采用后一种技术沉积1-甲基烟酰胺氯(MNA)Cl的光学不透明晶体层,用于随后的紫外线照射实验。1-甲基烟酰胺阳离子(MNA)Cl可作为假想的与NAD(P)+相关的地外烟酰胺氧化还原辅助因子的模型。在UV (λ≥224 nm)照射下,(MNA)Cl发生分解,但在~ 14天后停止,大部分材料完好无损。这种行为归因于晶体表面的光产物层的屏蔽作用,并且可以用一阶有界衰变模型进行动力学描述。这种“自我保存”可能会提高某些有机生物特征的生存能力,前提是它们形成足够厚的(不透明的)层或晶体。合成石膏(CaSO4·2H2O)或盐石(NaCl)的存在对(MNA)Cl的紫外分解动力学参数影响很小。
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引用次数: 0
Coexistence of O-band polarization-entangled photons with C-band classical channels in a dynamically reconfigurable metropolitan fiber network. 动态可重构城域光纤网络中o波段偏振纠缠光子与c波段经典信道的共存。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-09-28 DOI: 10.1364/OL.608372
Thomas Rieser, Hsuan-Hao Lu, Shane Andrewski, Mael Flament, Maximilian Schulz, Marc Geitz, Oliver Holschke, Mehdi Namazi, Matheus Sena

We present polarization entanglement distribution over an operator-owned, metropolitan-scale fiber network, employing standard wavelength-division multiplexing components to achieve coexistence of O-band photons and C-band classical light. First, we demonstrate dynamic path switching by alternating between 15-km and 30-km deployed fiber loops, enabled by automated polarization compensation achieving sub-second recovery and time-averaged CHSH S-values exceeding 2.65 over 21 hours. We then assess the impact of co-propagating 100-Gbit/s C-band classical signals by varying launch powers up to 6 dBm. Finally, by combining path switching and classical co-propagation, we achieve stable entanglement distribution over 30 km of deployed fiber, validating the feasibility of hybrid quantum-classical transmission and paving the way for entanglement-based quantum networking on existing metropolitan infrastructure.

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引用次数: 0
RGB color constancy from multispectral images via hierarchical physics-injection and spectral augmentation. 通过分层物理注入和光谱增强从多光谱图像的RGB色彩常数。
IF 1.5 3区 物理与天体物理 Q3 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-09-11 DOI: 10.1364/JOSAA.592076
Peng Zhang, Long Ma, Kaida Xiao, Changjun Li

Computational color constancy (CCC) aims to recover the canonical appearance of scenes, yet current spectral-based approaches are hindered by the scarcity of hyperspectral data. This limitation compels reliance on suboptimal two-stage strategies, restricting the potential of deep learning. To overcome this, we propose a physically accurate spectral data augmentation strategy that expands the training set five-fold using real-world illuminants. Leveraging this, we introduce the Hierarchical Physics-Injection Network (HPI-Net). Experiments demonstrate that, within the full-multispectral-input setting, HPI-Net achieves a 20% reduction in mean recovery angular error relative to the strongest compared baseline, validating the effectiveness of our end-to-end physics-injection architecture.

计算色彩恒常性(CCC)旨在恢复场景的规范外观,但目前基于光谱的方法受到高光谱数据稀缺的阻碍。这种限制迫使我们依赖于次优的两阶段策略,限制了深度学习的潜力。为了克服这个问题,我们提出了一种物理精确的光谱数据增强策略,该策略使用现实世界的光源将训练集扩展了五倍。利用这一点,我们引入了分层物理注入网络(HPI-Net)。实验表明,在全多光谱输入设置下,相对于最强基线,HPI-Net的平均恢复角误差降低了20%,验证了端到端物理注入架构的有效性。
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引用次数: 0
Wavefront-preserved thermal-optical design of a high-heat-load grazing-incidence X-ray mirror. 高热负荷掠入射x射线反射镜的波前保存热光学设计。
IF 1.5 3区 物理与天体物理 Q3 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-10-08 DOI: 10.1364/JOSAA.611622
Zhen Wang, Fang Liu, Weizhen Lei, Xiaohao Dong, Yuzhu Wang, Yajun Tong

High-repetition-rate X-ray free-electron laser facilities impose stringent requirements on the thermal stability and wavefront preservation of beamline mirrors. In this work, a coupled thermal-optical optimization method is developed for the first reflective mirror of the FEL-III beamline at the SHINE facility under an absorbed heat load of up to 11.12 W at a photon energy of 15 keV and a repetition rate of 200 kHz, with a peak absorbed power density of 0.0718 W/mm2. The cooling length and cooling-groove distance from the optical surface are jointly optimized, and their effects on residual height error, slope error, and focal-plane Strehl ratio are evaluated using thermal-structural analysis and X-ray tracing. The results show that the mirror performance is governed by the coupled cooling geometry rather than by either parameter alone. Compared with the initial full-length cooling design, the optimized design reduces the RMS residual height error by 73.7% and the RMS slope error by 68.9%. The system-level Strehl ratio increases from 0.45 to 0.993, exceeding the target value of 0.96, while stray-light features are suppressed and a compact focal intensity distribution is recovered at the sample plane. These results demonstrate that deformation-based thermal optimization, when combined with system-level X-ray tracing, provides an effective thermal-optical design route for preserving wavefront quality in high-heat-load grazing-incidence X-ray optical systems.

高重复率的x射线自由电子激光设备对光束线反射镜的热稳定性和波前保存提出了严格的要求。本文研究了在吸收热负荷高达11.12 W、光子能量为15 keV、重复频率为200 kHz、峰值吸收功率密度为0.0718 W/mm2的情况下,SHINE设施中FEL-III光束线的第一面反射镜的热光学耦合优化方法。通过热结构分析和x射线示踪,对冷却长度和冷却槽距光学表面的距离进行了优化,并评价了它们对残余高度误差、斜率误差和焦平面Strehl比的影响。结果表明,反射镜的性能受耦合冷却几何形状的影响,而不是单独受任何一个参数的影响。与初始全程冷却设计相比,优化后的RMS残差高度误差降低了73.7%,RMS斜率误差降低了68.9%。系统级Strehl比从0.45增加到0.993,超过了目标值0.96,杂散光特征被抑制,在样品平面上恢复了紧凑的焦强度分布。这些结果表明,基于变形的热优化与系统级x射线示踪相结合,为保持高热负荷掠入射x射线光学系统的波前质量提供了有效的热光学设计途径。
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引用次数: 0
Diode-pumped Yb:LLF laser with multi-watt SESAM mode locking and broad CW tuning. 二极管泵浦Yb:LLF激光器,具有多瓦SESAM模式锁定和宽连续波调谐。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-08-26 DOI: 10.1364/OL.609311
Serdar Okuyucu, Umit Demirbas, Jelto Thesinga, Mikhail Pergament, Franz X Kärtner

We demonstrate a diode-pumped Yb:LLF laser that combines multi-watt semiconductor saturable absorber mirror (SESAM) mode locking with record continuous-wave (CW) tuning. Using a compact cavity pumped by a single-emitter 10 W multimode diode at 960 nm, the laser provides up to 3.2 W CW output with a tuning range from 996 to 1073 nm and a slope efficiency of 42%. In mode-locked operation, it delivers up to 2.8 W of average power with 180 fs pulses (10.9 nJ at 257.5 MHz) in a high-power regime, and up to 570 mW with 110 fs pulses (2.6 nJ at 214.1 MHz) in a short-pulse regime. Compared to previous work, this represents more than an order-of-magnitude increase in usable mode-locked power and pulse energy together with a substantially extended CW tuning span, and we outline straightforward routes to further broaden the tuning, shorten the pulses, and scale the usable average power. Taken together with earlier results on Yb:YLF, these findings indicate that Yb:LLF can serve as a competitive sister host and a strong candidate for future high-power and cryogenic Yb-based laser and amplifier studies.

我们展示了一种二极管泵浦的Yb:LLF激光器,它结合了多瓦半导体可饱和吸收镜(SESAM)模式锁定和记录连续波(CW)调谐。该激光器采用紧凑的腔体,由一个10w的单发射极多模二极管泵浦,波长为960 nm,可提供高达3.2 W的连续输出,调谐范围为996 ~ 1073 nm,斜率效率为42%。在模式锁定操作中,在高功率工作状态下,180 fs脉冲(10.9 nJ, 257.5 MHz)可提供高达2.8 W的平均功率,在短脉冲工作状态下,110 fs脉冲(2.6 nJ, 214.1 MHz)可提供高达570 mW的平均功率。与之前的工作相比,这意味着可用的锁模功率和脉冲能量增加了一个数量级以上,同时大幅度延长了连续波调谐跨度,我们概述了进一步扩大调谐、缩短脉冲和扩大可用平均功率的直接途径。结合Yb:YLF的早期研究结果,这些发现表明Yb:LLF可以作为具有竞争力的姊妹宿主,并成为未来高功率和低温Yb基激光器和放大器研究的强有力候选者。
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引用次数: 0
Second-harmonic injection for nonlinear phase-ripple suppression in four-step fringe projection profilometry. 四步条纹投影轮廓术中二阶谐波注入抑制非线性相位纹波。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-09-30 DOI: 10.1364/OL.613374
Haitao Wu, Yiping Cao, Yu Zhang, Jinlong Li, Kai Yang, Jianping Peng, Yingying Wan

Projector-camera nonlinearity produces carrier-locked phase ripple in four-step fringe projection profilometry. We introduce second-harmonic injection, whose coefficient controls the third-fifth harmonic imbalance through nonlinear intermodulation, while the injected harmonic is rejected by ideal four-step demodulation. A two-stage spatial-reuse calibration selects the coefficient directly from measured ripple, evaluating 22 candidates using eight images. Across eight independent reference-plane projection-capture repetitions, the method achieved a phase RMSE of 0.00617 ± 0.00009 rad (mean ± sample standard deviation), compared with 0.02243 ± 0.00038 rad without correction. Sculpture-model measurements further demonstrated ripple suppression on a complex surface. The method provides efficient active predistortion for repeated four-step profilometry under a stable, calibrated response.

在四步条纹投影轮廓术中,投影-相机非线性产生载波锁相纹波。引入二次谐波注入,其系数通过非线性互调控制三、五次谐波不平衡,而注入的谐波被理想的四步解调抑制。两阶段空间重用校准直接从测量的纹波中选择系数,使用8张图像评估22个候选值。在8个独立的参考平面投影捕获重复中,该方法的相位RMSE为0.00617±0.00009 rad(平均值±样本标准差),而未经校正的相位RMSE为0.02243±0.00038 rad。雕塑模型测量进一步证明了波纹在复杂表面上的抑制作用。该方法在稳定的校准响应下为重复四步轮廓测量提供了有效的主动预失真。
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引用次数: 0
Sub-1 K measurement of silicon thermal expansion with a Fabry-Perot cavity-stabilized laser. 用法布里-珀罗腔稳定激光器测量低于1 K的硅热膨胀。
IF 3.3 2区 物理与天体物理 Q2 OPTICS Pub Date : 2026-11-01 Epub Date: 2026-07-16 DOI: 10.1364/OL.607376
Pierre Roset, Yara Hariri, Rémi Meyer, Jacques Millo, Clément Lacroûte, Samuel Margueron, Yann Kersalé, Jonathan Gillot

Advances in optical atomic clocks and the forthcoming redefinition of the SI second are pushing for ultra-stable lasers with extremely low short-term instability and predictable drift. Cryogenic silicon Fabry-Perot cavities are promising candidates for this purpose. Here, we report the lowest operating temperature achieved for a laser-stabilized Fabry-Perot cavity, and the most precise measurement of the silicon coefficient of thermal expansion (CTE) to date. Measurements were performed from 655 mK to 16 K using a laser stabilized to an 18 cm single-crystal silicon cavity. Below 1 K, the CTE lies in the 10-13K-1 range, reaching a minimum of 3.5(4)×10-13K-1 at 655 mK. We also develop a model based on Debye and Einstein approaches that reproduces the measured CTE in this range. These results show reliable ultra-stable operation at sub-Kelvin temperatures and open new perspectives for optical clocks and fundamental physics tests.

光学原子钟的进步和即将到来的国际单位制秒的重新定义正在推动超稳定激光器具有极低的短期不稳定性和可预测的漂移。低温硅法布里-珀罗腔是这一目的的有希望的候选者。本文报道了激光稳定法布里-珀罗腔的最低工作温度,以及迄今为止最精确的硅热膨胀系数(CTE)测量。测量范围为655 mK至16 K,使用激光稳定在18cm单晶硅腔内。在1k以下,CTE位于10-13K-1范围内,在655 mK时达到最低3.5(4)×10-13K-1。我们还开发了一个基于Debye和爱因斯坦方法的模型,该模型可以再现该范围内测量到的CTE。这些结果显示了在亚开尔文温度下可靠的超稳定运行,为光学时钟和基础物理测试开辟了新的视角。
{"title":"Sub-1 K measurement of silicon thermal expansion with a Fabry-Perot cavity-stabilized laser.","authors":"Pierre Roset, Yara Hariri, Rémi Meyer, Jacques Millo, Clément Lacroûte, Samuel Margueron, Yann Kersalé, Jonathan Gillot","doi":"10.1364/OL.607376","DOIUrl":"https://doi.org/10.1364/OL.607376","url":null,"abstract":"<p><p>Advances in optical atomic clocks and the forthcoming redefinition of the SI second are pushing for ultra-stable lasers with extremely low short-term instability and predictable drift. Cryogenic silicon Fabry-Perot cavities are promising candidates for this purpose. Here, we report the lowest operating temperature achieved for a laser-stabilized Fabry-Perot cavity, and the most precise measurement of the silicon coefficient of thermal expansion (CTE) to date. Measurements were performed from 655 mK to 16 K using a laser stabilized to an 18 cm single-crystal silicon cavity. Below 1 K, the CTE lies in the 10<sup>-13</sup>K<sup>-1</sup> range, reaching a minimum of 3.5(4)×10<sup>-13</sup>K<sup>-1</sup> at 655 mK. We also develop a model based on Debye and Einstein approaches that reproduces the measured CTE in this range. These results show reliable ultra-stable operation at sub-Kelvin temperatures and open new perspectives for optical clocks and fundamental physics tests.</p>","PeriodicalId":19540,"journal":{"name":"Optics letters","volume":"51 21","pages":"6042-6045"},"PeriodicalIF":3.3,"publicationDate":"2026-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149299541","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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