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Influence of Gold Nanoparticles on the Generation of Reactive Oxygen Species under Shock Impact on an Aqueous Solution 金纳米颗粒对水溶液冲击下活性氧生成的影响
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.3103/S1541308X25600266
I. A. Shcherbakov, I. V. Baimler, S. V. Gudkov, A. O. Dikovskaya, M. V. Dubinin, E. V. Karmanova, M. O. Klimenko, V. I. Pustovoi, M. B. Rebezov, K. V. Sergienko, M. A. Sevost’yanov, A. V. Simakin

Shock impact is found to affect the properties of droplets of synthesized colloidal nanoparticles falling on a solid surface. Luminescence of droplets, caused by their impact with a solid surface, is detected. It is established that the luminescence intensity increases with increasing the droplet fall height, nanoparticle concentration, and concentration of molecular oxygen dissolved in the liquid. It is revealed that the reactive oxygen species generation under a shock impact is enhanced by the presence of nanoparticles in the solution.

研究发现,冲击冲击会影响合成的胶体纳米颗粒滴落在固体表面上的性能。由于液滴撞击固体表面而产生的发光被检测到。结果表明,发光强度随液滴下落高度、纳米粒子浓度和液体中溶解的分子氧浓度的增加而增加。结果表明,纳米粒子的存在促进了激波冲击下活性氧的生成。
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引用次数: 0
Study of the Properties of an Aqueous Solution of Polar Organics at a Specific Point in Experiments on Measuring the Adiabatic Compressibility and on Dynamic Light Scattering 绝热压缩率和动态光散射实验中极性有机物水溶液特定点性质的研究
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.3103/S1541308X25700220
N. F. Bunkin, L. M. Sabirov, D. I. Semenov, F. R. Ismailov, Sh. A. Kadirov

The results of temperature and concentration experimental studies of the intensity ratio in the scattered light fine structure components (Landau–Placzek ratio) in γ-picoline aqueous solutions are presented. A significant increase in the Landau–Placzek ratio is revealed in a narrow concentration range near the so-called specific point. The specific point corresponds to the polar organic solvent concentration at which formation of molecular aggregates of water and organic component occurs. The sizes of these aggregates were estimated in experiments on measuring the adiabatic compressibility and on dynamic light scattering; the results of measurements according to these independent techniques are in very good agreement. It is concluded that the technique based on measuring the adiabatic compressibility in the gigahertz range of sound frequencies is efficient for estimating the sizes of spatial inhomogeneities at the specific point.

给出了γ-吡啶水溶液中散射光精细结构组分的强度比(Landau-Placzek比)的温度和浓度实验研究结果。在所谓的特异点附近的一个狭窄浓度范围内,朗多-普莱泽克比值显著增加。特定的点对应于极性有机溶剂的浓度,在此浓度下,水和有机组分的分子聚集体形成。在绝热压缩实验和动态光散射实验中对这些聚集体的大小进行了估计;根据这些独立技术的测量结果是非常一致的。结果表明,在千兆赫声频范围内测量绝热压缩率的方法可以有效地估计特定点上空间非均匀性的大小。
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引用次数: 0
Manipulation of Coherent Optical Phenomena and the Generation of Orbital Angular Momentum-Based Four-Wave Mixing Signal Using Structured Light 利用结构光处理相干光学现象和产生基于轨道角动量的四波混频信号
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.3103/S1541308X25600242
Samim Akhtar, Jayanta K. Saha, Md. Mabud Hossain

We study various coherent optical properties, e.g., two-photon electromagnetically induced transparency (EIT) and three-photon electromagnetically induced transparency and absorption (TPEIT/TPEIA), in a four-level ladder (Ξ)-type system of 87Rb atoms, where the probe and control fields are Gaussian-shaped laser beams and the pump field is structured laser beam. Additionally, the generated four-wave mixing (FWM) signal has been studied. Interestingly, it is found that the generated FWM signal is spatially structured along with the azimuthal phase, which carries the orbital angular momentum (OAM) of light. It is also observed that the coherent optical responses (EIT, TPEIT/TPEIA, and FWM signals) can be manipulated by utilizing the OAM number of the pump beam as a control knob.

在四能级阶梯(Ξ)型87Rb原子体系中,以高斯形激光束为探测场和控制场,以结构激光束为泵浦场,研究了双光子电磁感应透明(EIT)和三光子电磁感应透明与吸收(TPEIT/TPEIA)等相干光学性质。此外,对产生的四波混频(FWM)信号进行了研究。有趣的是,我们发现产生的FWM信号在空间上与方位角相一致,它携带光的轨道角动量(OAM)。利用泵浦光束的OAM数作为控制旋钮,可以对相干光响应(EIT、TPEIT/TPEIA和FWM信号)进行控制。
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引用次数: 0
Parametric Down-Conversion of Near-IR Laser Radiation into the Mid-IR Range Using Nonlinear LiGaSe2 and LiGaS2 Crystals with Antireflection Microstructures 具有增反射微结构的非线性LiGaS2和LiGaS2晶体将近红外激光辐射参数下转换为中红外
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-09-04 DOI: 10.3103/S1541308X25600308
S. N. Smetanin, P. D. Kharitonova, A. G. Papashvili, L. I. Isaenko, A. F. Kurus, A. P. Yelisseyev, A. A. Goloshumova, A. A. Bushunov, A. A. Teslenko, V. A. Lazarev, M. K. Tarabrin

The LiGaSe2 and LiGaS2 crystals with antireflection microstructures are comparatively tested as frequency down-converters into the mid-infrared range (4874 nm) in a two-stage optical parametric oscillator with a single cavity under intracavity pumping with a Nd:YLF laser with a wavelength of 1047 nm and a pulse duration of 25 ns. The first stage of optical parametric oscillation in the KTiOAsO4 crystal produces two-micron radiation with wavelengths of 1724 and 2668 nm at a pulse energy of up to 2 mJ. In the second stage of conversion, the LiGaS2 crystal with antireflection microstructures compared to LiGaSe2 with antireflection microstructures proves to be more efficient despite the lower effective nonlinearity coefficient, which can be explained by the higher optical quality of the crystal. The energy of the radiation pulse with a wavelength of 4874 nm reaches the level of 100 nJ.

利用波长为1047 nm、脉冲持续时间为25 ns的Nd:YLF激光器,在单腔双级光学参量振荡器中,对具有抗反射微结构的LiGaSe2和LiGaS2晶体进行了中红外(4874 nm)降频测试。KTiOAsO4晶体的光学参量振荡的第一阶段产生波长为1724和2668 nm的两微米辐射,脉冲能量高达2 mJ。在转换的第二阶段,与具有增透微结构的LiGaS2晶体相比,具有增透微结构的LiGaS2晶体的效率更高,尽管有效非线性系数更低,这可以解释为晶体的光学质量更高。波长为4874 nm的辐射脉冲能量达到100 nJ的水平。
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引用次数: 0
Partially Diffusive Structural Mechanism of the Transitions between Ices III and V III型和V型冰过渡的部分扩散结构机制
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X2570013X
E. A. Zheligovskaya

It is shown that the structures of ices III and V can be divided into nearly identical chiral layers. In achiral ice V, the right-handed enantiomorphic layers alternate with the left-handed ones. Chiral ice III consists of only right-handed or only left-handed layers. A structural mechanism preserving these layers is proposed for the transitions between ices III and V. This mechanism is partially diffusive. The possibility for the proposed structural mechanism to provide the experimentally observed high transition rate is discussed. Small structural units of crystal ices are shown to change regularly with increasing pressure in the sequence III, V, and VI. Such small structures formed by water molecules can be present in liquid near the crystallization curve.

结果表明,冰III和冰V的结构可以划分为几乎相同的手性层。在非手性冰V中,右手对纯层与左手对纯层交替存在。手性冰III只由右手或左手层组成。在冰III和冰v之间的过渡中,提出了一种保留这些层的结构机制,这种机制部分是扩散的。讨论了所提出的结构机制提供实验观察到的高跃迁速率的可能性。晶体冰的小结构单元在III、V和VI序列中随着压力的增加而有规律地变化。这种由水分子形成的小结构可以出现在结晶曲线附近的液体中。
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引用次数: 0
Paradox of Radiant Power and the Issue of Localized Currents 辐射功率悖论与局域电流问题
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25600047
Yu. A. Akimov

Two fundamental questions of modern theoretical physics—the paradox of radiant power and the issue of localized currents—are discussed in the paper. The radiant power paradox is the dilemma of whether electrodynamic systems radiate power outward or not. Mathematical analysis of the microscopic Maxwell equations describing excitation and propagation of electromagnetic fields shows that the total radiant power should be zero, whereas many classical problems considering localized currents argue the opposite. The paradox is resolved by proving limited applicability of localized-current models to calculations of energy and momentum characteristics of electromagnetic fields. The nonzero value of the total radiant power for these currents turns out to be the localized current approximation error, while the true radiant power value is always zero for physically consistent excitation currents. On the basis of analysis of physically consistent currents, an improved model of localized currents is proposed that enables physically consistent description of electromagnetic fields from the viewpoint of their energy and momentum characteristics but at the expense of causality violation in the external current-free region.

本文讨论了现代理论物理学的两个基本问题——辐射功率悖论和定域电流问题。辐射功率悖论是电动力系统是否向外辐射功率的困境。对描述电磁场激发和传播的微观麦克斯韦方程组的数学分析表明,总辐射功率应为零,而许多考虑局域电流的经典问题则相反。通过证明局域电流模型在电磁场能量和动量特性计算中的有限适用性,解决了这一悖论。这些电流的总辐射功率的非零值是局部电流近似误差,而物理一致励磁电流的真实辐射功率值始终为零。在分析物理一致电流的基础上,提出了一种改进的局域电流模型,该模型能够从能量和动量特征的角度对电磁场进行物理一致的描述,但代价是在外无电流区域违反因果关系。
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引用次数: 0
Random Pinning Models: Phase Transitions in Aqueous Solutions of Colloidal Particles 随机钉钉模型:胶体颗粒水溶液中的相变
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700116
E. N. Tsiok, S. A. Bobkov, E. E. Tareyeva, Yu. D. Fomin, V. N. Ryzhov

Self-assembly of colloidal particles may occur, for example, both under the action of external fields and due to the presence of pinning centers in a real experimental system. Of particular interest is the formation of condensed phases from an aqueous solution of colloidal particles on a substrate in an external rotating magnetic field. Substrate defects (for example, the substrate roughness) are of great importance in an experiment. These defects can act as pinning centers, to which colloidal particles are strongly attracted; this may lead to a change in the melting scenario. Changing the field rotation angle, one can obtain different colloidal structures. At small rotation angles, the system behaves like a two-dimensional system with a purely repulsive soft-disk potential, whereas at large angles it is similar to a generalized Lennard-Jones (LJ) system with an (nm)-potential. When the field rotates in the plane of the system, its phase diagram qualitatively resembles that of a classical model system with a LJ pair potential. The results of the computer simulation of a two-dimensional system with a LJ potential in the presence of Gauss pinning are discussed in the context of its influence on the phase diagram and melting scenario. It is shown that random pinning with a Gauss potential leads to an increase in the hexatic phase range; formation of dense clusters near pinning centers, which reduce the average effective density of the system; and a change in the melting scenario.

胶体粒子的自组装可能发生,例如,在外场的作用下,由于在实际的实验系统中存在钉住中心。特别令人感兴趣的是,在外部旋转磁场中,胶体颗粒的水溶液在衬底上形成凝聚相。衬底缺陷(例如,衬底粗糙度)在实验中是非常重要的。这些缺陷可以作为钉住中心,胶体粒子被强烈吸引到那里;这可能导致融化情景的变化。改变磁场旋转角度,可以得到不同的胶体结构。在较小的旋转角度下,系统表现得像一个具有纯排斥软盘势的二维系统,而在较大的旋转角度下,它类似于一个具有(nm)势的广义Lennard-Jones (LJ)系统。当场在系统平面上旋转时,其相图定性地类似于具有LJ对势的经典模型系统的相图。本文讨论了具有LJ势的二维体系在高斯钉钉作用下的计算机模拟结果,并讨论了其对相图和熔化情况的影响。结果表明,高斯势随机钉住导致六相范围增大;在钉钉中心附近形成密集的团簇,降低了体系的平均有效密度;以及融化情况的改变。
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引用次数: 0
Optimization of the Characteristics of Fiber-Optic Fabry–Perot Interferometer Mirrors in Measurement Systems Using Broadband Radiation 宽带辐射测量系统中光纤法布里-珀罗干涉仪反射镜特性的优化
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700165
I. G. Likhachev

The fiber-optic Fabry–Perot interferometer (FPI) has been analyzed to determine its reflection and transmission coefficients providing the maximum useful signal in a high-precision scheme for measuring the FPI length. It is shown that the traditionally applied criterion, which is aimed at achieving the maximum visibility of the interference pattern, is not applicable in this scheme. An adequate criterion is proposed, and an analysis based on it is presented. The optimal characteristics of the FPI mirrors are calculated taking into account the diffraction effects. The result of the study is a set of simple analytical relations necessary for designing mirrors in the form of thin films deposited on the fiber end face. In particular, the possibility of implementing a desired mirror on the fiber end in the form of a single-layer dielectric film is investigated and its characteristics are obtained.

对光纤法布里-珀罗干涉仪(FPI)进行了分析,确定了其反射系数和透射系数,为高精度测量FPI长度提供了最大有用信号。结果表明,传统的干涉图可见性准则在该方案中不适用。提出了一个适当的判据,并在此基础上进行了分析。在考虑衍射效应的情况下,计算了FPI反射镜的最佳特性。研究的结果是一组简单的分析关系,这是设计以薄膜形式沉积在光纤端面的反射镜所必需的。特别地,研究了在光纤端以单层介质膜的形式实现所需反射镜的可能性,并获得了其特性。
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引用次数: 0
Investigation of the Influence of pH and Temperature of an Aqueous Solution on the Stability of the Gold Nanoparticles–Lysozyme Protein System by Optical Methods 光学方法研究水溶液pH和温度对金纳米颗粒-溶菌酶蛋白体系稳定性的影响
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700141
E. A. Molkova, T. A. Matveeva, I. V. Baimler, R. M. Sarimov, S. V. Gudkov, A. S. Dorokhov, A. Yu. Izmailov

Gold nanoparticles are widely used in spectroscopy for detecting/studying substances in biological media. Such particles in biological objects inevitably interact with proteins, which obviously affects the functions and properties of the nanomaterial. The influence of external conditions on the interaction of nanoparticles with proteins in the aqueous phase has still remained little studied. In this paper we investigate the influence of temperature and pH of the medium on the interaction of lysozyme protein with gold nanoparticles in aqueous solutions. It is found that the temperature of the medium affects the size of aggregates of gold nanoparticles with protein at pH 7.5 of the aqueous solutions. It is found that lysozyme prevents protein aggregation at acidic pH values; with an increase in temperature, gold particles with a lysozyme protein crown retain their size. The results of this study gain a deeper insight into the processes of interaction between enzymes and gold nanoparticles with a change in the solvent properties.

金纳米颗粒被广泛应用于光谱检测/研究生物介质中的物质。这些粒子在生物物体中不可避免地与蛋白质相互作用,这明显影响了纳米材料的功能和性能。外界条件对纳米颗粒与水相蛋白质相互作用的影响研究仍然很少。本文研究了温度和pH对溶菌酶蛋白与金纳米颗粒在水溶液中相互作用的影响。研究发现,在pH为7.5的水溶液中,介质温度对金纳米粒子与蛋白质聚集体的大小有影响。发现溶菌酶在酸性pH值下阻止蛋白质聚集;随着温度的升高,具有溶菌酶蛋白冠的金颗粒保持其大小。本研究的结果对酶与金纳米颗粒的相互作用过程以及溶剂性质的变化有了更深入的了解。
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引用次数: 0
Short-Period Background Internal Waves in the Kara Sea in the Water Area near Cape Zhelaniya 热拉尼亚角附近海域喀拉海短周期背景内波
IF 1.1 4区 物理与天体物理 Q3 PHYSICS, MULTIDISCIPLINARY Pub Date : 2025-07-20 DOI: 10.3103/S1541308X25700207
Yu. V. Nazarenko, D. D. Sidorov, A. V. Zimin, E. I. Svergun, V. G. Petnikov, I. O. Kopyshov, I. E. Kozlov

The results from field measurements of hydrological characteristics of the Kara Sea water during the expedition on the research vessel Professor Molchanov in the summer of 2024 are reported. Vertical oscillations of temperature at fixed depths (vertical liquid oscillations) caused by short-period background internal waves are detected in the thermocline using extended “yo-yo” CTD profiling synchronous with an independently operating buoy-mounted thermistor chain. Their considerable effect on the vertical temperature distribution is shown. Energy spectra of the above-mentioned oscillations are obtained. It is demonstrated that the region under consideration near Novaya Zemlya can be regarded as a region where background internal waves quite often occur. The statistical characteristics of the fields of these waves are compared to those of similar wave fields on the Atlantic shelf and near the Kamchatka shore.

报告了2024年夏天莫尔查诺夫教授号科考船对喀拉海水水文特征的实地测量结果。利用扩展的“悠悠”CTD剖面与独立运行的浮标热敏电阻链同步,在温跃层中探测到由短周期背景内波引起的固定深度温度垂直振荡(垂直液体振荡)。它们对垂直温度分布有相当大的影响。得到了上述振荡的能谱。结果表明,所考虑的靠近新地岛的区域可以看作是一个经常发生背景内波的区域。将这些波场的统计特征与大西洋陆架和堪察加海岸附近的类似波场进行了比较。
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引用次数: 0
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Physics of Wave Phenomena
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