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Memristors Empowering Next-Generation Human-Computer Interaction 记忆电阻器助力下一代人机交互
IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 Epub Date: 2026-09-12 DOI: 10.1002/adfm.78446
Jinlong He, Bo Yang, Bai Sun, Qi Chen, Chuncai Kong, Zelin Cao, Kaikai Gao, Mengna Wang, Longhui Fu, Kun Wang, Teng Wu, Songling Wang, Ye Tang, Jinyou Shao

With the continuous advancement of artificial intelligence, human-computer interaction (HCI) is evolving toward intelligent perception, collaborative decision-making, and natural integration. However, the physical separation of memory and computing units in traditional von Neumann architecture poses critical bottlenecks in terms of power consumption and latency, which limits its ability to meet the requirements of next-generation HCI systems. Memristors, with their unique advantages of in-memory computing, synaptic plasticity emulation, and multi-physical responsiveness, have emerged as a key enabling technology for brain-inspired perception and interaction systems. This article systematically reviews the latest research progress of memristors in intelligent perception and neuromorphic systems for next-generation HCI. First, starting from the material system, performance regulation, and application adaptation are analyzed. Second, the strategy of memristors in device design and integration architecture is discussed. Furthermore, the biomimetic perception system based on memristors is emphasized, demonstrating its integration capability at the hardware level of brain-inspired perception information processing. Finally, it systematically summarizes the research achievements of memristors in the field of HCI applications and discusses the key challenges currently faced. Looking forward, this review suggests that memristors are expected to provide a solid foundation for building high-performance, low-power, and biocompatible next-generation HCI systems.

本文系统综述了记忆电阻器在下一代人机交互(HCI)智能感知和神经形态系统中的最新研究进展。展望未来,本文认为忆阻器有望为构建高性能、低功耗和生物相容性的下一代HCI系统提供坚实的基础。
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引用次数: 0
Harnessing Defect Engineered Multiferroic Catalysts for Cascade Responsive Microwave and Sonodynamic Therapy in Osteomyelitis 利用缺陷工程多铁催化剂进行级联响应微波和声动力治疗骨髓炎
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79253
Xuxu Chen,Jing Ren,Quanheng Yu,Ziwei Zhao,Shichang Liu,Xinhua Yin,Liang Yan,Ming Yang
Schematic illustration of the fabrication of RP/Mn-BFO hydrogel microspheres and their sequential therapeutic mechanism for bacterial osteomyelitis under microwave/ultrasound dual-field stimulation. The dual-field stimulation triggers Mn-BFO nanosheets to generate heat and burst ROS for sterilization, while the sustained release of RP-EVs promotes macrophage M2 polarization and osteogenic repair.
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引用次数: 0
Screening-Effect-Driven Growth of Large-Area High-Quality COF Films with Wavelength-Dependent Photochromism 具有波长依赖光变色的大面积高质量COF薄膜的筛选效应驱动生长
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79334
Furui Luo,Mengfan Xu,Xinping Cao,Jun Zhang,Lili Zhao,Ying Chu,Shengnan Guo,Xueying Wang,Ying-yan Hu,Yongping Zhu,Song Wang
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引用次数: 0
Targeting ALOX15 with a ROS-Responsive Lipid Nanoparticle for the Treatment of Allergic Conjunctivitis and Its Comorbidity Dry Eye Disease 靶向ALOX15的ros反应性脂质纳米颗粒治疗过敏性结膜炎及其合并症干眼病
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79285
Zhi Wang,Huimin Shan,Rui Yao,Jingchen Li,Xiaohua Yu,Xiaomei Tang,Xibo Ma,Ming Wang,Yong Tao,Xiaojun Wang
This study identifies ALOX15 as a shared core therapeutic target for allergic conjunctivitis (AC) and dry eye disease (DED). We subsequently construct a ROS-responsive lipid nanoparticle system loaded with siALOX15 (rLNP@siALOX15). rLNP@siALOX15 simultaneously suppresses inflammation and lipid peroxidation, showing favorable efficacy and biosafety in AC, DED, and comorbid models, representing a promising ocular surface therapeutic candidate.
本研究确定ALOX15是过敏性结膜炎(AC)和干眼病(DED)的共同核心治疗靶点。随后,我们构建了负载siALOX15的ros响应脂质纳米颗粒系统(rLNP@siALOX15)。rLNP@siALOX15同时抑制炎症和脂质过氧化,在AC、DED和合并症模型中显示出良好的疗效和生物安全性,是一种有前景的眼表治疗候选者。
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引用次数: 0
Realizing Reversible Lithium Anode at Micro-Nanoscale by a Gradient Ion-Electron Conductive Framework (Adv. Funct. Mater. 86/2026) 用梯度离子-电子导电骨架函数实现微纳级可逆锂阳极。板牙。86/2026)
IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.78668
Hong Liao, Yueqi Zhang, Wenjun Sun, Mengyue Liu, Shengpu Rao, Weishan Cao, Zhihong Lu, Nannan Guo, Jin Niu, Feng Wang

Gradient Framework

The gradient ion-electron conductive framework effectively achieves non-surface and dendrite-free Li deposition with high capacity. The Li metal batteries assembled with anodes modified by the framework exhibit excellent performance and show potential for powering electric vehicles. In the Research Article DOI: (10.1002/adfm.77338), Mengyue Liu, Nannan Guo, Jin Niu, Feng Wang, and co-workers establishe new design of three-dimensional framework for high-performance Li metal batteries.

梯度离子-电子导电框架有效地实现了高容量无表面、无枝晶的锂沉积。由该框架修饰的阳极组装的锂金属电池表现出优异的性能,并显示出为电动汽车提供动力的潜力。在研究文章DOI:(10.1002/adfm。77338),刘梦跃,郭楠楠,牛瑾,王峰,和同事建立了高性能锂金属电池的三维框架的新设计。
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引用次数: 0
Programming of Hierarchical Noncovalent Interactions Enables Thermoplastic Elastomers With Ultrahigh Mechanical Strength and Dynamic Stability 分层非共价相互作用的编程使热塑性弹性体具有超高的机械强度和动态稳定性
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79309
Xinshu Sun,Yucheng Hu,Baohua Guo,Jiaxin Shi,Jun Xu
Multiscale simulations guide the modular design of polyurethane hard segments to program hierarchical noncovalent interactions before synthesis. π–π stacking provides directional anchoring that promotes cooperative hydrogen bonding and stabilizes hard domains. The resulting thermoplastic elastomer combines 99.6 MPa tensile strength with resistance to heat, chemicals, and stress relaxation, offering a predictive route to robust soft materials.
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引用次数: 0
Rigid–Flexible Coupled Si3N4 Nanoribbon Aerogels With Carbon–Ceramic Hot-Face Armor for Oxidation-Resistant Thermal Protection Stable to 1600°C in Air 具有碳陶瓷热面装甲的刚柔耦合氮化硅纳米带气凝胶,用于抗氧化热防护,在空气中稳定到1600°C
IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 Epub Date: 2026-09-12 DOI: 10.1002/adfm.78440
Dongfang Xu, Lei Feng, Qiang Song, Qiangang Fu

Reconciling ultralight compliance with ultrahigh-temperature oxidation resistance under one-sided heating remains a key challenge for ceramic aerogels in extreme thermal protection systems (TPS). Here we report a spatially programmed rigid–flexible aerogel, locally impregnated ZrO2/SiO2/C–Si3N4 nanoribbon aerogel (L-ZSC-SNRA), fabricated by bidirectional freeze-casting and stepwise localized impregnation of polycarbosilane (PCS) and Zr-containing PCS precursors followed by pyrolysis. The ≈30 mg cm−3 monolith is functionally graded, decoupling hot-face protection from cold-face compliance by integrating a multiphase ZrO2/SiO2/C hot-face armor with a porous elastic Si3N4 skeleton. Consequently, L-ZSC-SNRA achieves 98% recoverability at 60% strain with stable 1000-cycle compression and retains ≈83% recoverability after single-sided static oxidation in air at 1600°C. It exhibits low thermal conductivity from 25°C–1000°C (38.6–105.2 mW m−1 K−1) and strong flame shielding under a ≈1500°C torch, limiting the cold-side temperature to 218.1°C for a 10-mm slab after 10 min. Notably, the thermal-conductivity increase at 1000°C after the 1600°C static oxidation is only 6.8%, evidencing robust high-temperature thermal-transport stability. This work overcomes the key trade-off between ultralight compliance and ultrahigh-temperature oxidation durability, demonstrating a scalable locally graded coating–architecture strategy for oxidizing extremes relevant to TPS.

一种刚柔耦合的氮化硅纳米带气凝胶具有致密的碳陶瓷热面装甲,用于极端热防护。通过集成独特的结构梯度,它提供了出色的热屏蔽1500°C火焰冲击,并在1600°C暴露后完美保持其宏观压缩弹性,为航空航天热防护系统提供了一个强大的材料平台。
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引用次数: 0
Electrostatic Superlattices Beyond 1:1 Stoichiometry 超过1:1化学计量的静电超晶格
IF 19.9 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 Epub Date: 2026-08-10 DOI: 10.1002/adfm.77545
Binay P. Nayak, Prapti Kakkar, Wesley P. Korba, Honghu Zhang, Wenjie Wang, Surya K. Mallapragada, Alex Travesset, David Vaknin
<p>Exotic nanoparticle superstructures can be accessed by harnessing nanoparticle softness and charge regulation, features often viewed as obstacles to structural control. Here, we show that regulated charge mismatch in polymer-grafted nanoparticles enables the assembly of high-stoichiometry cubic superlattices. By co-tuning grafting density, particle size, and bulk composition, we realize ionic-lattice analogues, such as <span></span><math> <semantics> <msub> <mi>CaF</mi> <mn>2</mn> </msub> <annotation>${rm CaF}_2$</annotation> </semantics></math> and <span></span><math> <semantics> <mrow> <msub> <mi>Th</mi> <mn>3</mn> </msub> <mi>P</mi> </mrow> <annotation>${rm Th}_3{rm P}$</annotation> </semantics></math><span></span><math> <semantics> <msub> <mrow></mrow> <mn>4</mn> </msub> <annotation>$_4$</annotation> </semantics></math>, as well as single-component <span></span><math> <semantics> <msub> <mi>A</mi> <mn>3</mn> </msub> <annotation>${rm A}_3$</annotation> </semantics></math> and <span></span><math> <semantics> <msub> <mi>A</mi> <mn>7</mn> </msub> <annotation>${rm A}_7$</annotation> </semantics></math> superlattices without atomic counterparts. The <span></span><math> <semantics> <msub> <mi>A</mi> <mn>3</mn> </msub> <annotation>${rm A}_3$</annotation> </semantics></math> superlattice has recently been identified theoretically as a photonic band-gap lattice. These phases emerge from a 1:1 “parent” lattice when local charge neutrality cannot be satisfied, driving either progressive interstitial filling or reorganization into a larger basis. For instance, the systematic occupation of ZnS tetrahedral sites yields <span></span><math> <semantics> <msub> <mi>CaF</mi> <mn>2</mn> </msub> <annotation>${rm CaF}_2$</annotation> </semantics></math>, while ligand-swapping symmetry breaking converts CsCl into <span></span><math> <semantics> <msub> <mi>Th</mi> <mn>3</mn> </msub> <annotation>${rm Th}_3$</annotation>
通过利用纳米粒子的柔软性和电荷调节,可以获得奇特的纳米粒子超结构,这些特征通常被视为结构控制的障碍。在这里,我们发现在聚合物接枝的纳米颗粒中调节电荷不匹配使得高化学计量立方超晶格的组装成为可能。通过共调接枝密度、颗粒大小和体积组成,我们实现了离子晶格类似物,例如CaF 2$ {rm CaF}_2$和th3p ${rm Th}_3{rm P}$ 4$ _4$,以及无原子对应物的单组分a3 ${rm A}_3$和a7 ${rm A}_7$超晶格。a3 ${rm A}_3$超晶格最近在理论上被确定为光子带隙晶格。当局部电荷中性不能满足时,这些相就会从1:1的“母”晶格中出现,从而驱动渐进的间隙填充或重组成更大的基。例如,系统占据ZnS四面体位得到caf2 ${rm CaF}_2$;配体交换对称破缺将CsCl转化为th3 ${rm Th}_3$ p4 ${rm P}_4$。在加热时,组件表现出可逆的晶格收缩和明显的负热膨胀。此外,缺陷的能量惩罚随着纳米颗粒尺寸的增加而增加,促进了用于光子应用的高质量开放超晶格的可扩展生产。
{"title":"Electrostatic Superlattices Beyond 1:1 Stoichiometry","authors":"Binay P. Nayak,&nbsp;Prapti Kakkar,&nbsp;Wesley P. Korba,&nbsp;Honghu Zhang,&nbsp;Wenjie Wang,&nbsp;Surya K. Mallapragada,&nbsp;Alex Travesset,&nbsp;David Vaknin","doi":"10.1002/adfm.77545","DOIUrl":"https://doi.org/10.1002/adfm.77545","url":null,"abstract":"&lt;p&gt;Exotic nanoparticle superstructures can be accessed by harnessing nanoparticle softness and charge regulation, features often viewed as obstacles to structural control. Here, we show that regulated charge mismatch in polymer-grafted nanoparticles enables the assembly of high-stoichiometry cubic superlattices. By co-tuning grafting density, particle size, and bulk composition, we realize ionic-lattice analogues, such as &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CaF&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CaF}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; and &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;mrow&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;Th&lt;/mi&gt;\u0000 &lt;mn&gt;3&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;mi&gt;P&lt;/mi&gt;\u0000 &lt;/mrow&gt;\u0000 &lt;annotation&gt;${rm Th}_3{rm P}$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt;&lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mrow&gt;&lt;/mrow&gt;\u0000 &lt;mn&gt;4&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;$_4$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt;, as well as single-component &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;A&lt;/mi&gt;\u0000 &lt;mn&gt;3&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm A}_3$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; and &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;A&lt;/mi&gt;\u0000 &lt;mn&gt;7&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm A}_7$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; superlattices without atomic counterparts. The &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;A&lt;/mi&gt;\u0000 &lt;mn&gt;3&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm A}_3$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt; superlattice has recently been identified theoretically as a photonic band-gap lattice. These phases emerge from a 1:1 “parent” lattice when local charge neutrality cannot be satisfied, driving either progressive interstitial filling or reorganization into a larger basis. For instance, the systematic occupation of ZnS tetrahedral sites yields &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;CaF&lt;/mi&gt;\u0000 &lt;mn&gt;2&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm CaF}_2$&lt;/annotation&gt;\u0000 &lt;/semantics&gt;&lt;/math&gt;, while ligand-swapping symmetry breaking converts CsCl into &lt;span&gt;&lt;/span&gt;&lt;math&gt;\u0000 &lt;semantics&gt;\u0000 &lt;msub&gt;\u0000 &lt;mi&gt;Th&lt;/mi&gt;\u0000 &lt;mn&gt;3&lt;/mn&gt;\u0000 &lt;/msub&gt;\u0000 &lt;annotation&gt;${rm Th}_3$&lt;/annotation&gt;\u0000 ","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"36 86","pages":""},"PeriodicalIF":19.9,"publicationDate":"2026-10-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adfm.77545","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149258112","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-Loading Ag Single Atoms Anchored on MoS2 Nanosheet Aggregates Enable Synergistic Nitrate-to-Ammonia Electroconversion 锚定在MoS2纳米片聚集体上的高负载银单原子实现了硝酸盐到氨的协同电转化
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79368
Ming-Xuan Shi,Ying-Ying Meng,Ying-Xue Shi,Ze-Nong Zhang,Shu-Ni Li,Xuan Ai,Yu Chen
Atomically dispersed Ag sites on MoS2 create a favorable reaction environment for the electroreduction of nitrates. These sites enhance nitrate adsorption, stabilize NOx-derived intermediates, and direct active hydrogen to subsequent hydrogenation reactions rather than hydrogen evolution reactions. Ag-MoS2 nanosheet aggregates achieve high ammonia selectivity, ampere-level current density, a yield of 30.6 mg h−1 cm−2, and stable operation for up to 200 h.
{"title":"High-Loading Ag Single Atoms Anchored on MoS2 Nanosheet Aggregates Enable Synergistic Nitrate-to-Ammonia Electroconversion","authors":"Ming-Xuan Shi,Ying-Ying Meng,Ying-Xue Shi,Ze-Nong Zhang,Shu-Ni Li,Xuan Ai,Yu Chen","doi":"10.1002/adfm.79368","DOIUrl":"https://doi.org/10.1002/adfm.79368","url":null,"abstract":"Atomically dispersed Ag sites on MoS2 create a favorable reaction environment for the electroreduction of nitrates. These sites enhance nitrate adsorption, stabilize NOx-derived intermediates, and direct active hydrogen to subsequent hydrogenation reactions rather than hydrogen evolution reactions. Ag-MoS2 nanosheet aggregates achieve high ammonia selectivity, ampere-level current density, a yield of 30.6 mg h−1 cm−2, and stable operation for up to 200 h.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"17 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149266389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dynamic Supramolecular Cryptomaterials for Compositional Encoding and Mechanical Decryption 用于组合编码和机械解密的动态超分子密码材料
IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Pub Date : 2026-10-27 DOI: 10.1002/adfm.79360
Zhen Hu,Xingduo Chen,Jing Wang,Xiujuan Zhang,Junsong Wu,Luyao Xu,Lianbin Zhang,Jintao Zhu
Dynamic supramolecular cryptomaterials constructed from multi-component colloids and polymer matrix enable compositional encoding and mechanical decryption for a robust, high-density information storage and advanced anti-counterfeiting cryptographic paradigm. Compositional encoding conceals identity within a featureless matte precursor, while only mechanical decryption through a correct and prescribed mechanical key induces a periodic superstructure, yielding unique structural colors, further enabling high-capacity, high-security anti-counterfeiting.
{"title":"Dynamic Supramolecular Cryptomaterials for Compositional Encoding and Mechanical Decryption","authors":"Zhen Hu,Xingduo Chen,Jing Wang,Xiujuan Zhang,Junsong Wu,Luyao Xu,Lianbin Zhang,Jintao Zhu","doi":"10.1002/adfm.79360","DOIUrl":"https://doi.org/10.1002/adfm.79360","url":null,"abstract":"Dynamic supramolecular cryptomaterials constructed from multi-component colloids and polymer matrix enable compositional encoding and mechanical decryption for a robust, high-density information storage and advanced anti-counterfeiting cryptographic paradigm. Compositional encoding conceals identity within a featureless matte precursor, while only mechanical decryption through a correct and prescribed mechanical key induces a periodic superstructure, yielding unique structural colors, further enabling high-capacity, high-security anti-counterfeiting.","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"4 1","pages":""},"PeriodicalIF":19.0,"publicationDate":"2026-10-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"149266386","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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