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Climate impact of delayed carbon dioxide removal by a single emitting entity to compensate for their legacy emissions 单一排放实体为补偿其遗留排放而延迟二氧化碳去除的气候影响
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-10-01 Epub Date: 2026-10-12 DOI: 10.1016/j.ijggc.2026.104806
Tuvshinjargal Otgonbayar, Marco Mazzotti
Carbon dioxide removal (CDR) is increasingly recognized as a key component of climate strategies to offset unabatable residual emissions on the path to net zero. In recent years, corporations in particular have shown growing interest in using CDR to offset their historical or “legacy” emissions. However, the prevailing assumption that one tonne of CO2 removed today cancels a tonne emitted in the past neglects the temporal mismatch between emissions and removals, during which CO2 exerts a warming effect. This paper considers specific entities that emit a very small fraction of global emissions, have a net-zero carbon goal and pledge to compensate for their legacy emissions. It examines the effectiveness of such compensation through climate consequences of delayed CDR, arguing that a simple mass-balance approach may not be sufficient. Using a simplified linear climate model, we analyze the impact of the timing and rate of CDR deployment on two complementary climate metrics: peak surface temperature and abyssal ocean temperature anomaly, reflecting direct short-term and long-term cumulative impacts, respectively. Our results show that earlier CDR deployment, even at slower rates, yields a more favorable climate outcome than delayed, faster deployment. The analysis also reveals that removing more CO2 than was originally emitted can help mitigate the effects of delayed action, particularly for long-term climate impacts. These findings highlight the importance of accounting for temporal dynamics in climate mitigation strategies. Our work aims to inform corporate climate policies and encourage further scientific discourse on the dynamic effects of legacy emissions and legacy removals.
二氧化碳去除(CDR)越来越被认为是气候战略的关键组成部分,以抵消在实现净零排放的道路上无法抑制的剩余排放。近年来,企业尤其对使用CDR抵消其历史或“遗留”排放表现出越来越大的兴趣。然而,普遍的假设是,今天清除一吨二氧化碳抵消了过去排放的一吨二氧化碳,忽略了排放和清除之间的时间不匹配,在此期间二氧化碳会产生变暖效应。本文考虑了排放占全球排放量很小一部分、有净零碳目标并承诺补偿其遗留排放的特定实体。它通过延迟CDR的气候后果来检验这种补偿的有效性,认为简单的质量平衡方法可能是不够的。利用简化的线性气候模型,我们分析了CDR部署时间和速率对两个互补气候指标的影响:地表峰值温度和深海温度异常,分别反映了直接的短期和长期累积影响。我们的研究结果表明,较早部署CDR,即使速度较慢,也比延迟、快速部署产生更有利的气候结果。分析还表明,消除比最初排放更多的二氧化碳有助于减轻延迟行动的影响,特别是对长期气候影响。这些发现突出了在气候减缓战略中考虑时间动态的重要性。我们的工作旨在为企业气候政策提供信息,并鼓励对遗留排放和遗留清除的动态影响进行进一步的科学讨论。
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引用次数: 0
Geospatial allocation of biogenic CO2 supply and demand for CCUS in Finland: A scenario analysis 芬兰CCUS生物源CO2供需的地理空间分配:情景分析
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-10-01 Epub Date: 2026-10-06 DOI: 10.1016/j.ijggc.2026.104805
Onni Linjala, Lauri Kujanpää
This study examines the availability, infrastructure demand and supply costs of biogenic CO2 for carbon capture, utilization and storage (CCUS) in Finland. A heuristic geospatial allocation model that aims to minimize CO2 transport demand is developed to evaluate potential CO2 supply and hub configurations under policy-based CCUS deployment scenarios. The examined large industrial facilities in Finland emit 29 Mt of biogenic CO2 annually. Due to the lack of domestic geological storage capacity and the need for CO2 shipping, the model consistently forms CCS hubs near seaports adjacent to large emission sources. Within the scenarios and system boundary examined, centralized CCU hubs can reduce investments, but the cost benefit is largely offset by increased transport demand. Seasonally variable sources have higher specific investment costs when dimensioned for peak load but excluding such sources from a hub-based CCUS system appears to yield little or no economic advantage because the hub areas expand and transport demand increases. Across the scenarios examined, the levelized cost of CO2 supply, including capture, compression and transport to CCS hub ports or utilization sites, ranges from 79 to 95 €/tCO2. With a CO2 capture volume of 14.8 Mtpa, investments in CO2 supply infrastructure range from EUR 3.5 to 5.0 billion. For CO2 utilization capacities ranging from 3.7 to 11.1 Mtpa, investments in CO2 utilization and hydrogen production infrastructure range from EUR 3.6 to 9.5 billion. The findings provide insights into CCUS infrastructure planning in regions with abundant CO2 sources but limited domestic geological storage capacity.
本研究考察了芬兰用于碳捕获、利用和封存(CCUS)的生物源二氧化碳的可用性、基础设施需求和供应成本。开发了一种启发式地理空间分配模型,旨在最大限度地减少二氧化碳运输需求,以评估基于策略的CCUS部署场景下潜在的二氧化碳供应和枢纽配置。被调查的芬兰大型工业设施每年排放2900万吨生物二氧化碳。由于国内缺乏地质储存能力和二氧化碳运输的需要,该模型始终在靠近大型排放源的海港附近形成CCS中心。在研究的场景和系统边界内,集中式CCU枢纽可以减少投资,但成本效益在很大程度上被增加的运输需求所抵消。当考虑峰值负荷时,季节性可变源具有更高的特定投资成本,但从基于枢纽的CCUS系统中排除此类源似乎很少或根本没有经济优势,因为枢纽区域扩大和运输需求增加。在研究的所有情景中,二氧化碳供应的平准化成本,包括捕集、压缩和运输到CCS枢纽港口或利用地点,从79欧元到95欧元/吨二氧化碳不等。二氧化碳捕集量为1480万吨/年,二氧化碳供应基础设施的投资从35亿欧元到50亿欧元不等。二氧化碳利用能力为370万至11100万吨/年,二氧化碳利用和氢气生产基础设施的投资为36亿至95亿欧元。这一发现为二氧化碳来源丰富但国内地质储存能力有限的地区的CCUS基础设施规划提供了见解。
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引用次数: 0
From expert weighting to data-derived evidence: A leakage-safe, physics-motivated, uncertainty-aware machine-learning framework for CO₂ storage site screening in the Gulf of Mexico 从专家加权到数据证据:墨西哥湾CO₂储存场地筛选的泄漏安全、物理驱动、不确定性意识机器学习框架
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-10-01 Epub Date: 2026-10-07 DOI: 10.1016/j.ijggc.2026.104808
Amir Hossein Nazari, Mohammadali Ahmadi
Selecting where to permanently store CO₂ across the offshore Gulf of Mexico (GoM) is a high-stakes decision that precedes every well, requiring thousands of candidate grid blocks to be ranked from sparse, spatially correlated evidence. The prevailing approach, expert-weighted multi-criteria decision analysis (MCDA), encodes this choice in subjective, scenario-dependent weights that cannot be validated, quantify no uncertainty, and predict none of the physical reservoir properties, storage capacity and injectivity, that ultimately govern where CO₂ can be stored. Data-driven models promise objectivity, but naïve machine learning (ML) on spatial geoscience data silently leaks information across neighboring blocks, inflates reported accuracy, recycles the very score it should predict (circularity), and returns point estimates with no error bars. Using the 2,559-block NETL GoM screening dataset as the sole data source, we build a leakage-controlled pipeline: an anti-circularity raw-feature whitelist, physics-based interaction features, per-target leakage whitelists, and a single spatial-block split tuned to match the train/test distribution of every target. Six complementary spatial learners, a physics-motivated gradient-boosting stack, a graph neural network, a physics-informed network, a geospatial transformer, a tabular foundation model, and a Gaussian-process kriging model, predict storage capacity, injectivity, and a multiplicative storage-deliverability index, each wrapped in distribution-free conformal uncertainty and explained with a common SHAP protocol. The best learner reaches a test R2 of 0.98 on the composite suitability target under the original predictor set, and 0.89 under a stricter predictor set that additionally excludes two ordinal variables encoding part of that target's own containment-risk term; nominal 90% conformal intervals achieve empirical coverage of 0.83 to 0.95, and the data-derived suitability index reproduces the experts' geologic-storage rankings (quadratic-weighted κ up to 0.65). Because the composite target is constructed rather than observed, this figure quantifies learnability under leakage-safe spatial validation rather than validated storage performance. Where our ranking diverges from the expert screen, we show the divergence is driven by the weight carried by hydrocarbon-derived criteria rather than by superior storage quality, and we report it as a criterion-weighting diagnostic. The result is a reproducible, uncertainty-aware suitability surface for regional high-grading, intended to prioritize blocks for subsequent characterization rather than to initialize dynamic reservoir simulation.
选择在墨西哥湾(GoM)近海永久存储CO₂的位置是每口井之前的高风险决策,需要从稀疏的空间相关证据中对数千个候选网格区块进行排序。目前流行的方法是专家加权多标准决策分析(MCDA),该方法将这种选择编码为主观的、依赖于场景的权重,这些权重无法验证,无法量化不确定性,也无法预测最终决定二氧化碳储存位置的储层物理性质、储存能力和注入能力。数据驱动的模型承诺了客观性,但是naïve空间地球科学数据的机器学习(ML)会在相邻块之间悄悄地泄露信息,夸大报告的准确性,回收它应该预测的分数(圆度),并返回没有误差条的点估计。使用2,559块NETL GoM筛选数据集作为唯一数据源,我们构建了一个泄漏控制管道:反循环原始特征白名单,基于物理的交互特征,每个目标泄漏白名单,以及单个空间块分割,以匹配每个目标的训练/测试分布。六个互补的空间学习器,一个物理驱动的梯度增强堆栈,一个图神经网络,一个物理信息网络,一个地理空间转换器,一个表格基础模型和一个高斯过程克里格模型,预测存储容量,注入性和乘法存储交付能力指数,每个都包裹在无分布的保形不确定性中,并用一个通用的SHAP协议进行解释。在原始预测集下,最佳学习者在复合适宜性目标上的检验R2为0.98,在更严格的预测集下,在额外排除了编码目标自身包含风险项部分的两个有序变量的情况下,最佳学习者的检验R2为0.89;名义90%适形区间的经验覆盖率为0.83至0.95,数据衍生的适宜性指数再现了专家的地质存储排名(二次加权κ高达0.65)。由于复合目标是构建的而不是观察的,因此该图量化了泄漏安全空间验证下的可学习性,而不是经过验证的存储性能。如果我们的排名与专家筛选的结果有差异,我们会显示这种差异是由烃类衍生标准所占的权重驱动的,而不是由优越的储存质量驱动的,我们将其作为标准加权诊断报告。结果是一个可重复的、具有不确定性意识的区域高分级适用性曲面,旨在优先考虑区块进行后续表征,而不是初始化动态油藏模拟。
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引用次数: 0
Experimental study on the electrical resistivity characteristics of CO2 hydrate-bearing silty-clayey sediments under formation stress 地层应力作用下含CO2水合物粉砂质粘土沉积物电阻率特征试验研究
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-10-01 Epub Date: 2026-10-14 DOI: 10.1016/j.ijggc.2026.104811
Aowang Wang, Tingting Luo, Liwei Zhang, Xiang Sun, Tao Han, Zhen Zhang, Yanghui Li, Yongchen Song, Ye Zhang, Madhusudhan B N, Weihao Yang
Carbon Capture, Utilization, and Storage (CCUS) is a critical pathway for mitigating the global greenhouse effect. Sub-seabed CO2 sequestration, particularly through hydrate-based methods, offers immense potential due to the vast storage capacity and favorable thermodynamic conditions of marine sediments. However, the complex phase transitions and associated geomechanical deformations pose significant challenges for in-situ monitoring of CO2 evolution and reservoir stability. This study utilizes a triaxial-resistivity apparatus to investigate the electrical response of silty-clayey sediments during CO2 hydrate formation and subsequent deformation under varying saturations and effective stresses. Key findings indicate that resistivity is highly sensitive to temperature and pore fluid content, with a 10 % difference in initial water saturation leading to an 88 % variation in resistivity. Furthermore, hydrate morphology and residual water distribution significantly influence electrical signals, resulting in resistivity fluctuations of up to 853 Ω·m at identical saturation levels. Beyond phase identification, resistivity effectively reflects sediment consolidation and pore structure evolution during the shearing stage, exhibiting a non-linear correlation with applied stress. These results demonstrate the feasibility of resistivity-based monitoring for tracking CO2 dynamics and assessing the mechanical integrity of sub-seabed reservoirs, providing essential theoretical support for large-scale sequestration in the future.
碳捕获、利用与封存(CCUS)是缓解全球温室效应的重要途径。由于海洋沉积物具有巨大的储存能力和有利的热力学条件,海底下二氧化碳封存,特别是通过基于水合物的方法,提供了巨大的潜力。然而,复杂的相变和相关的地质力学变形给CO2演化和储层稳定性的原位监测带来了重大挑战。本研究利用三轴电阻率仪研究了粉质粘土沉积物在不同饱和度和有效应力下,在CO2水合物形成和随后变形过程中的电响应。关键发现表明,电阻率对温度和孔隙流体含量高度敏感,初始含水饱和度相差10 %,导致电阻率变化88 %。水合物形态和残余水分布对电信号影响显著,在相同饱和度下电阻率波动高达853 Ω·m。除相识别外,电阻率还能有效反映剪切阶段沉积物固结和孔隙结构演化,与外加应力呈非线性相关。这些结果证明了基于电阻率的监测方法在跟踪CO2动态和评估海底储层机械完整性方面的可行性,为未来大规模封存提供了必要的理论支持。
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引用次数: 0
Corrigendum to “Geochemical framework for CO2 mineralization in coastal aquifers: Lessons from the Coda Terminal project, Iceland” [International Journal of Greenhouse Gas Control 149 (2026) 104565] “沿海含水层CO2矿化的地球化学框架:来自冰岛Coda终端项目的经验教训”[国际温室气体控制学报,149 (2026):104565]
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-22 DOI: 10.1016/j.ijggc.2026.104759
Iwona Galeczka, Martin Voigt, Daniel Andres Duque Carrillo, Kjartan Marteinsson, Thomas Ratouis, Sandra Ósk Snæbjörnsdóttir, Fríða Jónsdóttir, Paula Fernández Acosta, Gunnar Hrafn Gunnarsson, Bergur Sigfússon, Jóhann Gunnarsson Robin, Sif Pétursdóttir, Salka Kolbeinsdóttir, Magnús Á. Sigurgeirsson, Helga M. Helgadóttir, Gunnlaug Ásgeirsdóttir, Ólafur Elínarson
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引用次数: 0
Characterization of the lower Palaeozoic regarding its CO2-storage potential in the Swedish sector of the Baltic Sea 波罗的海瑞典海域下古生代co2储存潜力的表征
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-28 DOI: 10.1016/j.ijggc.2026.104763
Mikael Erlström, Peter Dahlqvist, Jan-Erik Rosberg
Two cored boreholes were drilled in 2023 through the Cambro–Silurian succession on the southernmost part of the island of Gotland as part of a project coordinated by the Geological Survey of Sweden to assess the CO2-storage potential in the Cambrian sandstone reservoirs in the south Baltic Sea. The investigations were performed in cooperation with the Swedish national research infrastructure for scientific drilling “Riksriggen”. We describe and assess the drilling, geophysical wire-line logging, and stratigraphical, lithological, and petrophysical analysis of the Cambro–Silurian succession. The results are discussed with respect to the reservoir and sealing properties for CO2-storage. The results indicate that the Faludden sandstone, along with the overlying Ordovician and Silurian caprock interval meets the necessary requirements for CO2-storage. In contrast the Cambrian Viklau and När sandstone intervals display less favourable reservoir conditions due to high degree of cementation contributing to very low permeability. Formation integrity tests and laboratory analyses verify an Ordovician and Silurian caprock interval with high compressive strength and low permeability. This new information strengthens the judgement that CO2 storage is feasible in the Swedish sector of the Baltic Sea.
2023年,在哥特兰岛最南端的寒武纪-志留纪地层中钻了两个取心井,作为瑞典地质调查局协调的项目的一部分,以评估波罗的海南部寒武纪砂岩储层的二氧化碳储存潜力。这些调查是与瑞典国家科学钻探“Riksriggen”研究基础设施合作进行的。我们描述和评估了寒武-志留纪演替的钻井、地球物理电缆测井、地层、岩性和岩石物理分析。讨论了储层和封存co2的特性。结果表明,法卢登砂岩及其上覆的奥陶系和志留系盖层符合co2储集的必要条件。相比之下,寒武纪Viklau和När砂岩层段由于胶结程度高,渗透率非常低,因此储层条件不太有利。地层完整性测试和实验室分析验证了奥陶系和志留系盖层具有高抗压强度和低渗透率。这一新资料加强了在波罗的海瑞典海域储存二氧化碳是可行的判断。
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引用次数: 0
Integrated geostatistical and machine learning reservoir modeling for CO2 plume prediction and storage safety assessment 综合地质统计学和机器学习油藏建模,用于CO2羽流预测和储存安全性评估
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-30 DOI: 10.1016/j.ijggc.2026.104766
Muhammad Ali, Ning Wei, Ren Jiang, Wendong Wang, Keyao Lin, Chang Jia
Hybrid reservoir property modeling is important for reliable CO2 storage assessment, particularly in areas with limited well control and strong reservoir heterogeneity. This study presents a Hybrid Geostatistics and Machine Learning workflow, termed HyGEM, to generate high-resolution reservoir property models for CO2 geological storage applications. The workflow integrates upscaled well-log data, multi-attribute seismic volumes, geostatistical modeling, and supervised machine learning to predict petrophysical properties within a 3D reservoir grid. Arithmetic averaging is first applied to upscale well-log data to the simulation-grid scale, helping preserve volumetric consistency and reduce high-frequency noise. Several seismic attributes, including Instantaneous Bandwidth, RMS Amplitude, Sweetness, RGB, Semblance, and thin-bed indicators, are then used to describe stratigraphic and structural variations around the injection zone. Based on these inputs, the workflow generates 3D models of porosity, permeability, water saturation, volume of shale, bulk density, and pore pressure while preserving vertical layering and lateral heterogeneity. Validation results show strong agreement with original and upscaled well log data, with improved geological continuity compared to conventional stochastic and deterministic approaches. The predicted property grids are further applied in dynamic CO2 injection simulation, where the results indicate controlled plume migration within high permeability zones, effective caprock containment, stable geomechanical behavior, and no clear indication of caprock failure during injection. These results demonstrate that the HyGEM workflow provides a practical and reliable approach for reservoir characterization, CO2 plume prediction, and long-term storage safety assessment.
混合储层性质建模对于可靠的CO2储存评估非常重要,特别是在井控有限且储层非均质性强的地区。本研究提出了一种名为HyGEM的混合地质统计学和机器学习工作流程,为二氧化碳地质储存应用生成高分辨率储层属性模型。该工作流程集成了升级的测井数据、多属性地震数据、地质统计建模和监督机器学习,以预测三维储层网格内的岩石物理性质。算法平均首先应用于将测井数据提升到模拟网格尺度,有助于保持体积一致性并降低高频噪声。然后使用瞬时带宽、均数振幅、甜度、RGB、相似度和薄层指标等地震属性来描述注入带周围的地层和构造变化。基于这些输入,工作流生成孔隙度、渗透率、含水饱和度、页岩体积、体积密度和孔隙压力的3D模型,同时保留垂直分层和横向非均质性。验证结果与原始和升级后的测井数据非常吻合,与传统的随机和确定性方法相比,具有更好的地质连续性。将预测的性质网格进一步应用于动态CO2注入模拟,结果表明,在高渗透区域内,羽流运移受到控制,盖层得到有效遏制,地质力学行为稳定,并且在注入过程中没有明显的盖层破坏迹象。这些结果表明,HyGEM工作流程为储层表征、CO2羽流预测和长期储存安全性评估提供了实用可靠的方法。
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引用次数: 0
Mineral-controlled precipitation provenance dictates the mineral trapping-injectivity trade-off in sandstone CO2 storage 矿物控制的降水物源决定了砂岩CO2储存中矿物圈闭与注入的权衡关系
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-28 DOI: 10.1016/j.ijggc.2026.104764
Hongjin Yu, Yixuan Fang, Shiwei Wu, Ziyou Zhu, Huanxiang Gao, Quan Xie, Ranjith Pathegama Gamage, Zhaoyang Ma
Balancing mineral trapping with pore-network preservation remains a key challenge for CO2 storage in deep saline sandstones. Here, we propose a precipitation-provenance framework to distinguish carbonate recycling from silicate- and clay-fed net carbonate formation. Two tight sandstones, a calcite-cemented red sandstone (RS1) and a plagioclase/chlorite-rich grey sandstone (GS1), were reacted with scCO2-brine at 120°C and 30 MPa. Image-registered ESEM-MapsMin automated mineralogy, CT-resolved 3D pore-network analysis, and ICP-OES brine chemistry were integrated to track coupled dissolution-precipitation from grain to core scale. RS1 followed a carbonate-buffered recycling pathway, where calcite dissolution-reprecipitation and feldspar corrosion increased CT porosity from ∼2.0% to ∼5.5% but produced limited net mineral trapping. In contrast, GS1 showed silicate-fed carbonate formation: plagioclase and chlorite supplied Ca-Mg-Fe, increasing MapsMin-derived calcite abundance from near-zero to ∼13 wt%, while pore-wall coatings and local throat restriction moderated pore growth. We further distinguish likely in situ pore-wall carbonates from depressurization-related carbonates and drying-derived halite to avoid overestimating reservoir-condition trapping. Together, these results provide mechanistic criteria for screening sandstone storage formations and for designing pressure-management strategies that maximize mineral trapping while limiting adverse pore-network feedbacks.
平衡矿物捕获和孔隙网络保存仍然是深层含盐砂岩中二氧化碳储存的关键挑战。在这里,我们提出了一个降水-物源框架,以区分碳酸盐再循环与硅酸盐和粘土喂养的净碳酸盐地层。将两种致密砂岩,方解石胶结的红砂岩(RS1)和富含斜长石/绿泥石的灰色砂岩(GS1),在120℃和30 MPa的条件下与scco2盐水反应。集成了图像注册ESEM-MapsMin自动矿物学、ct分辨率3D孔隙网络分析和ICP-OES盐水化学,以跟踪从颗粒到岩心尺度的耦合溶解-沉淀。RS1遵循碳酸盐缓冲循环路径,方解石溶解-再沉淀和长石腐蚀使CT孔隙度从~ 2.0%增加到~ 5.5%,但产生有限的净矿物捕获。相比之下,GS1显示了由硅酸盐供养的碳酸盐地层:斜长石和绿泥石提供Ca-Mg-Fe,将mapsmin衍生的方解石丰度从接近零增加到~ 13wt %,而孔壁涂层和局部喉道限制减缓了孔的生长。我们进一步将可能的原位孔壁碳酸盐与减压相关的碳酸盐和干燥衍生的岩盐区分开来,以避免高估储层条件的圈闭。总之,这些结果为筛选砂岩储层和设计压力管理策略提供了机制标准,从而最大限度地捕获矿物,同时限制不利的孔隙网络反馈。
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引用次数: 0
A RU-Net-based surrogate study of sand tank experiments for CO2 storage capacity in composite confining systems 基于ru - net的复合围封系统CO2储存量砂罐试验替代研究
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-31 DOI: 10.1016/j.ijggc.2026.104765
Yun-Ting Chou, Hailun Ni, Hannah Lu
As global CO2 emissions rise, geological carbon storage remains a critical mitigation strategy. While traditional storage focuses on reservoirs with continuous caprocks, composite confining systems, comprised of discontinuous barriers, have recently emerged as promising alternatives due to their ability to inhibit leakage through heterogeneity. Existing assessments using physical sand tanks or commercial simulators are often computationally expensive or lack flexibility. In this work, we develop a full-field RU-Net-based surrogate model trained on simulation data to predict flow paths and retention capacity from various capillary entry pressure fields and injection locations. We demonstrate how the resulting computationally efficient and accurate surrogate model enables global sensitivity analysis of barrier geometry and injection optimization that would otherwise be expensive using physical experiments or full-physics simulations. Our results indicate that retention capacity cannot be attributed to any single geometric parameter and instead arise from interaction effects among barrier length, wing angle, and dip angle. Together, these results show that the full-field machine learning surrogate model can provide an efficient and practical decision-support tool for screening, sensitivity analysis, and injection design in heterogeneous geological carbon storage systems.
随着全球二氧化碳排放量的增加,地质碳储存仍然是一项关键的缓解策略。传统的储层侧重于连续盖层的储层,而由不连续屏障组成的复合围封系统由于其抑制非均质性渗漏的能力,最近成为了有希望的替代方案。现有的使用物理砂罐或商业模拟器的评估通常在计算上昂贵或缺乏灵活性。在这项工作中,我们开发了一个基于ru - net的全油田代理模型,该模型经过模拟数据的训练,可以预测不同毛细管入口压力场和注入位置的流动路径和截留能力。我们展示了由此产生的计算效率高且准确的替代模型如何实现屏障几何和注入优化的全局敏感性分析,否则使用物理实验或全物理模拟将是昂贵的。研究结果表明,截留能力不能归因于任何单一的几何参数,而是由障壁长度、翼角和倾角之间的相互作用决定的。总之,这些结果表明,全场机器学习代理模型可以为非均质地质储碳系统的筛选、敏感性分析和注入设计提供高效实用的决策支持工具。
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引用次数: 0
Screening of Austrian geological carbon and hydrogen storage options. Part I: Hydrocarbon fields 奥地利地质储碳储氢方案筛选。第一部分:油气田
IF 5.9 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2026-09-01 Epub Date: 2026-08-28 DOI: 10.1016/j.ijggc.2026.104754
Jakob Kulich, Holger Ott
The carbon capture and storage (CCS) potential in Austria remains to be elucidated as the country plans to lift its CO2 storage ban and permit geologic storage for hard-to-abate emitters. This study presents a static screening and assessment of Austria’s CCS and underground hydrogen storage (UHS) potential in hydrocarbon reservoirs. Using reported ultimate recoveries from oil and gas fields, CO2 storage capacities were estimated across 73 reservoirs. The results indicate a total static CCS capacity of 263 Mt (183–357 Mt, depending on efficiency factor variation) for pure CO2, which decreases to 151–293 Mt when high levels of impurities are considered. The five largest gas fields, with individual storage capacities exceeding 10 Mt, account for approximately 100 Mt of CCS capacity. Site-specific challenges in Austria’s largest hydrocarbon fields may include numerous abandoned boreholes, strong aquifer support, and competition with UHS. Storage efficiency factors and CO2 density variations significantly impact capacity estimates, particularly in reservoirs near the supercritical threshold. For UHS, the total theoretical storage capacity across suitable fields was calculated to be 55 TWh, with 21 TWh identified in operational underground gas storage sites. Competition between CCS and UHS technologies is anticipated in relatively large gas fields with overlapping suitability. While individual CO2 storage capacities in hydrocarbon fields are small compared to offshore saline aquifers, they offer advantages such as existing infrastructure, detailed reservoir characterization, and proximity to major emission sources. The identified CCS capacity could bridge crucial periods before CO2 export or saline aquifer storage becomes viable.
奥地利的碳捕获与封存(CCS)潜力仍有待阐明,因为该国计划解除其二氧化碳封存禁令,并允许对难以减排的排放者进行地质封存。本研究对奥地利油气储层中的CCS和地下储氢(UHS)潜力进行了静态筛选和评估。根据报告的油气田最终采收率,估计了73个储层的二氧化碳储存能力。结果表明,纯CO2的总静态CCS容量为263 Mt (183-357 Mt,取决于效率因子变化),当考虑高杂质水平时,该容量降至151-293 Mt。五个最大的气田,单个存储容量超过1000万吨,约占CCS容量的1亿吨。奥地利最大的油气田面临的具体挑战可能包括大量废弃井眼、强大的含水层支撑以及与UHS的竞争。储存效率因素和二氧化碳密度变化显著影响储层容量估算,特别是在超临界阈值附近的储层。对于UHS,计算出合适气田的总理论存储容量为55太瓦时,其中在运营的地下储气库中确定了21太瓦时。预计CCS和UHS技术将在具有重叠适用性的相对较大的气田中展开竞争。虽然与海上咸水含水层相比,油气油田的单个二氧化碳储存能力较小,但它们具有现有基础设施、详细的储层特征以及靠近主要排放源等优势。确定的CCS容量可以跨越二氧化碳出口或咸水层储存变得可行之前的关键时期。
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International Journal of Greenhouse Gas Control
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